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Osadchii, D. (author), Olivos Suarez, A.I. (author), Szécsényi, A. (author), Li, G. (author), Nasalevich, M. (author), Dugulan, A.I. (author), Serra Crespo, P. (author), Hensen, Emiel J M (author), Veber, Sergey L. (author), Fedin, Matvey V. (author), Sankar, Gopinathan (author), Pidko, E.A. (author), Gascon Sabate, J. (author)
Hybrid materials bearing organic and inorganic motifs have been extensively discussed as playgrounds for the implementation of atomically resolved inorganic sites within a confined environment, with an exciting similarity to enzymes. Here, we present the successful design of a site-isolated mixed-metal metal organic framework (MOF) that...
journal article 2018
document
Vollmer, I. (author), van der Linden, B. (author), Ould-Chikh, Samy (author), Aguilar-Tapia, Antonio (author), Yarulina, I. (author), Abou-Hamad, Edy (author), Sneider, Yuri G. (author), Olivos Suarez, A.I. (author), Hazemann, Jean-Louis (author), Kapteijn, F. (author), Gascon Sabate, J. (author)
The mechanism of methane activation on Mo/HZSM-5 is not yet fully understood, despite the great interest in methane dehydroaromatization (MDA) to replace aromatics production in oil refineries. It is difficult to assess the exact nature of the active site due to fast coking. By pre-carburizing Mo/HZSM-5 with carbon monoxide (CO), the MDA active...
journal article 2018
document
Osadchii, D. (author), Olivos Suarez, A.I. (author), Bavykina, A.V. (author), Gascon Sabate, J. (author)
Covalent triazine frameworks (CTFs) are porous organic materials promising for applications in catalysis and separation due to their high stability, adjustable porosity, and intrinsic nitrogen functionalities. CTFs are prepared by ionothermal trimerization of aromatic nitriles; however, multiple side reactions also occur under synthesis...
journal article 2017
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Sun, X. (author), Olivos Suarez, A.I. (author), Meijerink, Mark (author), Van Deelen, Tom (author), Ould-Chikh, Samy (author), Zečević, Jovana (author), de Jong, K.M. (author), Kapteijn, F. (author), Gascon Sabate, J. (author)
The development of synthetic protocols for the preparation of highly loaded metal nanoparticle-supported catalysts has received a great deal of attention over the last few decades. Independently controlling metal loading, nanoparticle size, distribution, and accessibility has proven challenging because of the clear interdependence between...
journal article 2017
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Bavykina, A.V. (author), Olivos Suarez, A.I. (author), Osadchii, D. (author), Valecha, R.R. (author), Franz, R.P.M. (author), Makkee, M. (author), Kapteijn, F. (author), Gascon Sabate, J. (author)
Cp∗-based catalyst for the...
journal article 2017
document
Sun, X. (author), Olivos Suarez, A.I. (author), Oar-Arteta Gonzalez, L. (author), Rozhko, E. (author), Osadchii, D. (author), Bavykina, A.V. (author), Kapteijn, F. (author), Gascon Sabate, J. (author)
A Co@N-doped carbon (Co@ NC) hybrid was synthesized by thermal decomposition of the metal–organic framework (MOF) ZIF-67 under N2 atmosphere. These hybrid materials exhibit outstanding catalytic activity and chemoselectivity for the conversion of a wide range of substituted nitroarenes to their corresponding anilines under relatively mild...
journal article 2017
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Garcia Santaclara, J. (author), Olivos Suarez, A.I. (author), du Fossé, Indy (author), Houtepen, A.J. (author), Hunger, J (author), Kapteijn, F. (author), Gascon Sabate, J. (author), van der Veen, M.A. (author)
The highly porous titanium based metal–organic framework NH2-MIL-125(Ti) has recently attracted significant attention in the field of photocatalysis as a promising material for H+ reduction. This work reveals charge transfer upon visible light illumination from this MOF to two different charge acceptors, as an alternative to sacrificial electron...
journal article 2017
document
Rogge, S.M.J. (author), Bavykina, A.V. (author), Hajek, Julianna (author), Garcia, H (author), Olivos Suarez, A.I. (author), Sepúlveda-Escribano, A. (author), Vimont, A. (author), Clet, G (author), Bazin, P. (author), Kapteijn, F. (author), Daturi, Marco (author), Ramos-Fernandez, E.V. (author), Llabres i Xamena, FX (author), Van Speybroeck, V (author), Gascon Sabate, J. (author)
Heterogeneous single-site catalysts consist of isolated, well-defined, active sites that are spatially separated in a given solid and, ideally, structurally identical. In this review, the potential of metal–organic frameworks (MOFs) and covalent organic frameworks (COFs) as platforms for the development of heterogeneous single-site catalysts is...
journal article 2017
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Goesten, M.G. (author), de Lange, M.F. (author), Olivos Suarez, A.I. (author), Bavykina, A.V. (author), Serra Crespo, P. (author), Krywka, C. (author), Bickelhaupt, F. M. (author), Kapteijn, F. (author), Gascon Sabate, J. (author)
Chemical clocks are often used as exciting classroom experiments, where an induction time is followed by rapidly changing colours that expose oscillating concentration patterns. This type of reaction belongs to a class of nonlinear chemical kinetics also linked to chaos, wave propagation and Turing patterns. Despite its vastness in occurrence...
journal article 2016
document
Dikhtiarenko, A. (author), Olivos Suarez, A.I. (author), Pustovarenko, O. (author), García-Granda, Santiago (author), Gascon Sabate, J. (author)
journal article 2016
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