Single-molecule sensing with nanopores and nanoslits

We start this thesis by exploring the question whether there is more to be done with solid-state nanopores, given the success of nanopores for DNA sequencing applications.

Direct Comparison of PdAu Alloy Thin Films and Nanoparticles upon Hydrogen Exposure

Nanostructured metal hydrides are able to efficiently detect hydrogen in optical sensors. In the literature, two nanostructured systems based on metal hydrides have been proposed for this purpose each with its own detection principle: continuous sub-100 nm thin films read out via optical reflectance/transmittance changes and nanoparticle arrays...

Core-Shell Plasmonic Nanohelices

We introduce core-shell plasmonic nanohelices, highly tunable structures that have a different response in the visible for circularly polarized light of opposite handedness. The glass core of the helices is fabricated using electron beam induced deposition and the pure gold shell is subsequently sputter coated. Optical measurements allow us...

Plasmonic nanoparticle films for solar cell applications fabricated by size-selective aerosol deposition

A soft deposition method for incorporating surface plasmon resonant metal nanoparticles within photovoltaic devices was studied. This self-assembly method provides excellent control over both nanoparticle size and surface coverage. Films of spherical Ag nanoparticles with diameter of ?100 nm were fabricated by depositing size-selected aerosols...

Cathodoluminescence Microscopy of Nanostructures on Transparent Substrates

Cathodoluminescence (CL), the excitation of light by an electron beam, has gained attention as an analysis tool for investigating the optical response of a structure, at a resolution that approaches that in electron microscopy, in the nanometer range. However, the application possibilities are limited because the use of transparent substrates,...

Enhancing the driving field for plasmonic nanoparticles in thin-film solar cells

The scattering cross-section of a plasmonic nanoparticle is proportional to the intensity of the electric field that drives the plasmon resonance. In this work we determine the driving field pattern throughout a complete thin-film silicon solar cell. Our simulations reveal that by tuning of the thicknesses of silicon and transparent conductive...

Plasmon-enhanced four-wave mixing by nanoholes in thin gold films

Nonlinear plasmonics opens up for wavelength conversion, reduced interaction/emission volumes, and nonlinear enhancement effects at the nanoscale with many compelling nanophotonic applications foreseen. We investigate nonlinear plasmonic responses of nanoholes in thin gold films by exciting the holes individually with tightly focused laser beams...

Improved light trapping in microcrystalline silicon solar cells by plasmonic back reflector with broad angular scattering and low parasitic absorption

We show experimentally that the photocurrent of thin-film hydrogenated microcrystalline silicon (?c-Si:H) solar cells can be enhanced by 4.5?mA/cm2 with a plasmonic back reflector (BR). The light trapping performance is improved using plasmonic BR with broader angular scattering and lower parasitic absorption loss through tuning the size of...

Top-down fabrication of plasmonic nanostructures for deterministic coupling to single quantum emitters

Metal nanostructures can be used to harvest and guide the emission of single photon emitters on-chip via surface plasmon polaritons. In order to develop and characterize photonic devices based on emitter-plasmon hybrid structures, a deterministic and scalable fabrication method for such structures is desirable. Here, we demonstrate deterministic...

Advanced Light Management Approaches for Thin-Film Silicon Solar Cells

Light management is important for improving the performance of thin-film solar cells. Advanced concepts of efficient light scattering and trapping inside the cell structures need to be investigated. An important tool for design and optimisation of the concepts present optical modelling and simulation. In the article a model of light scattering...

Enhanced terahertz emission from thin film semiconductor/metal interfaces

Terahertz light is electromagnetic radiation, similar to visible light. The photons that the terahertz light is comprised of carry a much smaller amount of energy compared to the visible light photons. Unlike visible light, terahertz light can pass through materials like plastic, cardboards, wood etc.; a very useful property which enables it to...

Rigorous simulations of emitting and non-emitting nano-optical structures

In the next decade, several applications of nanotechnology will change our lives. LED lighting is about to replace the common light bulb. The main advantages are its energy efficiency and long lifetime. LEDs can be much more efficient, when part of the emitted light that is currently trapped in the device, could be radiated out of the device....