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Homborg, A.M. (author), Mol, J.M.C. (author), Tinga, Tiedo (author)This paper for the first time treats the interpretation of electrochemical noise time-frequency spectra as an image classification problem. It investigates the application of a convolutional neural network (CNN) for deep learning image classification of electrochemical noise time-frequency transient information. Representative slices of these...journal article 2024
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Imani, Amin (author), Rahimi, E. (author), Lekka, Maria (author), Andreatta, Francesco (author), Magnan, Michele (author), Gonzalez Garcia, Y. (author), Mol, J.M.C. (author), Raman, R. K. Singh (author), Fedrizzi, Lorenzo (author), Asselin, Edouard (author)Mg and its alloys are promising biodegradable materials for orthopedic implants and cardiovascular stents. The first interactions of protein molecules with Mg alloy surfaces have a substantial impact on their biocompatibility and biodegradation. We investigate the early-stage electrochemical, chemical, morphological, and electrical surface...journal article 2024
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Li, Z. (author), Visser, Peter (author), Hughes, Anthony E. (author), Homborg, A.M. (author), Gonzalez Garcia, Y. (author), Mol, J.M.C. (author)The quest for novel alternatives to hexavalent-chromium-based corrosion inhibitors is of utmost significance and urgency. Strict international health and safety regulations, due to growing concerns regarding the impact of hexavalent chromium on human health and the environment, have pushed the commercial introduction of many alternative...journal article 2024
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Cornet, A.J. (author), Homborg, A.M. (author), Ravi Anusuyadevi, P. (author), 't Hoen-Velterop, L. (author), Mol, J.M.C. (author)Despite extensive research, eliminating hexavalent chromium-based inhibitors from aerospace coatings remains challenging due to a lack of understanding of coating degradation during aircraft service. This study addresses the issue by investigating the protective mechanisms and aging processes of chromate-containing coatings on aircraft...journal article 2024
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Liu, Tong (author), Chen, Zhuoyao (author), Yang, Jingzhi (author), Ma, Lingwei (author), Mol, J.M.C. (author), Zhang, Dawei (author)Machine learning is a powerful means for the rapid development of high-performance functional materials. In this study, we presented a machine learning workflow for predicting the corrosion resistance of a self-healing epoxy coating containing ZIF-8@Ca microfillers. The orthogonal Latin square method was used to investigate the effects of the...journal article 2024
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Özkan, C. (author), Sahlmann, Lisa (author), Feiler, Christian (author), Zheludkevich, Mikhail (author), Lamaka, Sviatlana (author), Sewlikar, Parth (author), Kooijman, A.M. (author), Taheri, P. (author), Mol, J.M.C. (author)Creating durable, eco-friendly coatings for long-term corrosion protection requires innovative strategies to streamline design and development processes, conserve resources, and decrease maintenance costs. In this pursuit, machine learning emerges as a promising catalyst, despite the challenges presented by the scarcity of high-quality...journal article 2024
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Mopon, M. (author), Mol, J.M.C. (author), Garcia, Santiago J. (author)Understanding how late an inhibitor can be released once corrosion initiated without compromising corrosion protection may help in developing more efficient anticorrosion coatings. We explored this idea through time-controlled Ce(NO<sub>3</sub>)<sub>3</sub> availability to AA2024-T3 immersed in 0.05 M NaCl. Ce(NO<sub>3</sub>)<sub>3</sub> was...journal article 2024
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Gao, Yu (author), Zhang, Jingru (author), Wang, Donglei (author), Fan, Jiaxin (author), Mol, J.M.C. (author), Wang, Fuhui (author), Zhang, Danni (author), Xu, Dake (author)Microbially influenced corrosion (MIC) of metals exerts a negative effect on the marine environment and causes a great loss of marine facilities. Corrosion prevention in an eco-friendly and sustainable way is a difficult problem to address, especially in the marine environment. In this work, Nocardiopsis dassonville, a corrosive bacteria...journal article 2024
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Michailidou, E. (author), Visser, P. (author), Mol, J.M.C. (author), Kosari, A. (author), Terryn, H.A. (author), Baert, K. (author), Gonzalez Garcia, Y. (author)The corrosion inhibiting effect of lithium carbonate has been studied over the pH range relevant for atmospheric corrosion conditions at the polymer/metal interface. It is demonstrated that lithium carbonate offers optimum corrosion protection under moderately alkaline conditions attributed to the formation of a protective layer identified as...journal article 2023
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Liu, M. (author), Zhu, Jia-Ning (author), Popovich, V. (author), Borisov, E. (author), Mol, J.M.C. (author), Gonzalez Garcia, Y. (author)Electrochemical tests and surface analysis measurements were performed to study the corrosion behavior in a 0.9 wt.% NaCl solution at 37 °C of three NiTi shape memory alloys fabricated by laser-powder bed fusion (L-PBF). The passive film characteristics and corrosion resistance of L-PBF NiTi showed different features as a function of their...journal article 2023
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Li, Z. (author), Homborg, A.M. (author), Gonzalez Garcia, Y. (author), Visser, Peter (author), Soleimani, M. (author), Mol, J.M.C. (author)The influence of ageing under ambient conditions on the corrosion protective behaviour of a lithium-based conversion layer on AA2024-T3 is studied in this work. Conversion layers aged at ambient conditions for relatively short times (0 h and 4 h), show an initial high degree of corrosion inhibition but a much lower protectiveness after the...journal article 2023
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Cutz, L. (author), Tiringer, U. (author), de Jong, W. (author), Mol, J.M.C. (author)Long transport distances and extended storage of biomass pellets especially in humid environments provide a suitable setting for enhanced degradation in the form of moisture sorption, cracking and attrition. We developed an optically transparent, low-cost and environmentally friendly coating to reduce moisture sorption and storage degradation...journal article 2023
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Rahimi, E. (author), Sanchis-Gual, Roger (author), Chen, Xiangzhong (author), Imani, Amin (author), Gonzalez Garcia, Y. (author), Asselin, Edouard (author), Mol, J.M.C. (author), Fedrizzi, Lorenzo (author), Pané, Salvador (author), Lekka, Maria (author)The last two decades have witnessed the emergence of micro- and nanoswimmers (MNSs). Researchers have invested significant efforts in engineering motile micro- and nanodevices to address current limitations in minimally invasive medicine. MNSs can move through complex fluid media by using chemical fuels or external energy sources such as...review 2023
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Putra, N.E. (author), Leeflang, M.A. (author), Klimopoulou, M. (author), Dong, J. (author), Taheri, P. (author), Huan, Z. (author), Fratila-Apachitei, E.L. (author), Mol, J.M.C. (author), Chang, J. (author), Zhou, J. (author), Zadpoor, A.A. (author)The development of biodegradable Fe-based bone implants has rapidly progressed in recent years. Most of the challenges encountered in developing such implants have been tackled individually or in combination using additive manufacturing technologies. Yet not all the challenges have been overcome. Herein, we present porous FeMn-akermanite...journal article 2023
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Liu, M. (author), Zhu, Jia-Ning (author), Popovich, V. (author), Borisov, E. (author), Mol, J.M.C. (author), Gonzalez Garcia, Y. (author)Electrochemical tests and surface analysis were applied to study the corrosion behavior and passive film characteristics of three-dimensional-printed NiTi shape memory alloys fabricated by laser-powder bed fusion (L-PBF) in artificial saliva at 37 °C. The passivity of L-PBF NiTi shows to be influenced by the process parameters and resulting...journal article 2023
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Aghaeian, S. (author), Norouzi, F. (author), Sloof, W.G. (author), Mol, J.M.C. (author), Bottger, A.J. (author)The parabolic growth rate constant (k<sub>p</sub>) of high-temperature oxidation of steels is predicted via a data analytics approach. Four machine learning models including Artificial Neural Networks, Random Forest, k-Nearest Neighbors, and Support Vector Regression are trained to establish the relations between the input features ...journal article 2023
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Meeusen, M. (author), van Dam, J.P.B. (author), Madelat, N. (author), Jalilian, E. (author), Wouters, B. (author), Hauffman, T. (author), Van Assche, G. (author), Mol, J.M.C. (author), Hubin, A. (author), Terryn, H.A. (author)In this work, a new finite element modelling (FEM) approach is followed to model spatiotemporally resolved water uptake in organic coatings. To this aim, we start from a physical model, where not only Fickian diffusion of water is taken into account but also the adsorption/desorption reaction of water on the polymer matrix. Starting from a...journal article 2023
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Aghaeian, S. (author), Brouwer, J.C. (author), Sloof, W.G. (author), Mol, J.M.C. (author), Bottger, A.J. (author)Since the oxidation reactions in the process of steel production occur in harsh conditions (i.e., high temperatures and gas atmospheres), it is practically impossible to observe in situ the compositional changes in the steel and the formed oxide scale. Hence, a coupled thermodynamic-kinetic numerical model is developed that predicts the...journal article 2023
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Ma, Jinbo (author), Dai, Jiaxin (author), Guo, Xin (author), Fu, Dongmei (author), Ma, Lingwei (author), Keil, Patrick (author), Mol, J.M.C. (author), Zhang, Dawei (author)Following the construction of a dataset of cross-category corrosion inhibitors at different concentrations based on 1241 data from 184 research papers, a performance prediction model incorporating 2D–3D molecular graph representation and corrosion inhibitor concentration information was established. This model was shown to effectively predict...journal article 2023
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Rahimi, E. (author), Kim, Donghoon (author), Offoiach, Ruben (author), Sanchis-Gual, Roger (author), Chen, Xiang Zhong (author), Taheri, P. (author), Gonzalez Garcia, Y. (author), Mol, J.M.C. (author), Fedrizzi, Lorenzo (author), Pané, Salvador (author), Lekka, Maria (author)Functional oxide nanoparticles are extensively utilized in the last decades for biomedical purposes due to their unique functional properties. Nevertheless, their biodegradation mechanism by biological species, particularly by proteins at oxide/protein interfaces, still remains limited. Here, a systematic approaches is provided to investigate...journal article 2023