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Corral-Pérez, Juan José (author), Copéret, Christophe (author), Urakawa, A. (author)
Silica-supported silver nanoparticles exhibit outstanding efficiency in the CO<sub>2</sub> hydrogenation to methyl formate in the presence of methanol under high pressure. Here, we show that ZrO<sub>2</sub> and Al<sub>2</sub>O<sub>3</sub> supports significantly increase the catalyst activity, in line with their higher Lewis acidity. The...
journal article 2019
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Corral-Pérez, Juan José (author), Billings, Amelia (author), Stoian, Dragos (author), Urakawa, A. (author)
Continuous synthesis of formic acid and methyl formate via CO<sub>2</sub> hydrogenation is demonstrated using a molecular iridium complex stably immobilized on a solid covalent triazine framework (CTF) under high-pressure conditions. Compared to formic acid synthesis, methyl formate synthesis is advantageous to enhance the selectivity and...
journal article 2019