Searched for: author%3A%22Savenije%2C+T.J.%22
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Jöbsis, Huygen J. (author), Caselli, V.M. (author), Askes, Sven H.C. (author), Garnett, Erik C. (author), Savenije, T.J. (author), Rabouw, Freddy T. (author), Hutter, Eline M. (author)
Cs<sub>2</sub>AgBiBr<sub>6</sub> (CABB) has been proposed as a promising nontoxic alternative to lead halide perovskites. However, low charge carrier collection efficiencies remain an obstacle for the incorporation of this material in optoelectronic applications. In this work, we study the optoelectronic properties of CABB thin films using...
journal article 2021
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Zhao, J. (author), Caselli, V.M. (author), Bus, M. (author), Boshuizen, B. (author), Savenije, T.J. (author)
Wide-band-gap perovskites such as methylammonium lead bromide (MAPB) are promising materials for tandem solar cells because of their potentially high open-circuit voltage, which is yet still far below the maximum limit. The relatively short charge-carrier lifetimes deduced from time-resolved photoluminescence (TRPL) measurements seem in...
journal article 2021
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Lin, Yuze (author), Li, Tao (author), Liu, Ye (author), Bahrami, Behzad (author), Guo, Dengyang (author), Fang, Yanjun (author), Shao, Yuchuan (author), Wang, Qi (author), Savenije, T.J. (author)
A long photoluminescence decay lifetime has been regarded as a generic indication of long charge carrier recombination lifetime in semiconductors such as metal halide perovskites (MHPs), which have shown tremendous success in solar cells. Here, we report that MHP polycrystalline films with extrinsic metal ions have a very long charge...
journal article 2021
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Felter, K.M. (author), Fravventura, Maria C. (author), Koster, Emma (author), Abellon, R.D. (author), Savenije, T.J. (author), Grozema, F.C. (author)
In this contribution we demonstrate a solid-state approach to triplet-triplet annihilation upconversion for application in a solar cell device in which absorption of near-infrared light is followed by direct electron injection into an inorganic substrate. We use time-resolved microwave photoconductivity experiments to study the injection of...
journal article 2020
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Caselli, V.M. (author), Wei, Z. (author), Ackermans, M.M. (author), Hutter, E.M. (author), Ehrler, Bruno (author), Savenije, T.J. (author)
To further understand the optoelectronic properties of metal halide perovskites, we investigate sub-bandgap absorption in methylammonium lead iodide (MAPbI3) films. Charge carrier dynamics are studied using time-resolved microwave conductivity measurements using sub-bandgap excitation. From changes in the decay dynamics as a function of...
journal article 2020
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Caselli, V.M. (author), Fischer, Mathias (author), Meggiolaro, Daniele (author), Mosconi, Edoardo (author), De Angelis, Filippo (author), Stranks, Samuel D. (author), Baumann, Andreas (author), Dyakonov, Vladimir (author), Hutter, E.M. (author), Savenije, T.J. (author)
Recently, several studies have investigated dielectric properties as a possible origin of the exceptional optoelectronic properties of metal halide perovskites (MHPs). In this study we investigated the temperature-dependent dielectric behavior of different MHP films at different frequencies. In the gigahertz regime, dielectric losses in...
journal article 2019
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Guo, Dengyang (author), Andaji Garmaroudi, Zahra (author), Abdi-Jalebi, Mojtaba (author), Stranks, Samuel D. (author), Savenije, T.J. (author)
The highest reported efficiencies of metal halide perovskite (MHP) solar cells are all based on mixed perovskites, such as (FA,MA,Cs)Pb(I<sub>1-x</sub>Br<sub>x</sub>)<sub>3</sub>. Despite demonstrated structural changes induced by light soaking, it is unclear how the charge carrier dynamics are affected across this entire material family....
journal article 2019
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Guo, Dengyang (author), Caselli, V.M. (author), Hutter, E.M. (author), Savenije, T.J. (author)
While the power conversion efficiency of metal halide perovskite (MHP) solar cells has increased enormously, the open-circuit voltage, V <sub>oc</sub> , is still below the conceivable limit. Here, we derive the Fermi level splitting, μ <sub>F</sub> , for various types of noncontacted MHPs, which sets a limit for their achievable V <sub>oc<...
journal article 2019
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Muscarella, Loreta A. (author), Hutter, E.M. (author), Sanchez, Sandy (author), Dieleman, Christian D. (author), Savenije, T.J. (author), Hagfeldt, Anders (author), Saliba, Michael (author), Ehrler, Bruno (author)
Growing large, oriented grains of perovskite often leads to efficient devices, but it is unclear if properties of the grains are responsible for the efficiency. Domains observed in SEM are commonly misidentified with crystallographic grains, but SEM images do not provide diffraction information. We study methylammoinium lead iodide (MAPbI<sub...
journal article 2019
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Wei, Z. (author), Guo, Dengyang (author), Thieme, J. (author), Katan, Claudine (author), Caselli, V.M. (author), Even, Jacky (author), Savenije, T.J. (author)
Despite intense research into the optoelectronic properties of metal halide perovskites (MHPs), sub-bandgap absorption in MHPs remains largely unexplored. Here we recorded two-photon absorption spectra of MHPs using the time-resolved microwave conductivity technique. A two-step upward trend is observed in the two-photon absorption spectrum...
journal article 2019
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Andaji-Garmaroudi, Zahra (author), Abdi-Jalebi, Mojtaba (author), Guo, Dengyang (author), Macpherson, Stuart (author), Sadhanala, Aditya (author), Tennyson, Elizabeth M. (author), Ruggeri, Edoardo (author), Anaya, Miguel (author), Savenije, T.J. (author)
Mixed-halide lead perovskites have attracted significant attention in the field of photovoltaics and other optoelectronic applications due to their promising bandgap tunability and device performance. Here, the changes in photoluminescence and photoconductance of solution-processed triple-cation mixed-halide (Cs<sub>0.06</sub>MA<sub>0.15</sub...
journal article 2019
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Felter, K.M. (author), Caselli, V.M. (author), Gunbas, D.D. (author), Savenije, T.J. (author), Grozema, F.C. (author)
Two of the key parameters that characterize the usefulness of organic semiconductors for organic or hybrid organic/inorganic solar cells are the mobility of charges and the diffusion length of excitons. Both parameters are strongly related to the supramolecular organization in the material. In this work we have investigated the relation...
journal article 2019
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Hutter, E.M. (author), Gelvez Rueda, M.C. (author), Bartesaghi, D. (author), Grozema, F.C. (author), Savenije, T.J. (author)
Recently, halide double perovskites (HDPs), such as Cs<sub>2</sub>AgBiBr<sub>6</sub>, have been reported as promising nontoxic alternatives to lead halide perovskites. However, it remains unclear whether the charge-transport properties of these materials are as favorable as for lead-based perovskites. In this work, we study the mobilities of...
journal article 2018
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Abdi-Jalebi, Mojtaba (author), Andaji-Garmaroudi, Zahra (author), Cacovich, Stefania (author), Stavrakas, Camille (author), Philippe, Bertrand (author), Richter, Johannes M. (author), Alsari, Mejd (author), Booker, Edward P. (author), Hutter, E.M. (author), Savenije, T.J. (author)
Metal halide perovskites are of great interest for various high-performance optoelectronic applications. The ability to tune the perovskite bandgap continuously by modifying the chemical composition opens up applications for perovskites as coloured emitters, in building-integrated photovoltaics, and as components of tandem photovoltaics to...
journal article 2018
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Hutter, E.M. (author), Savenije, T.J. (author)
The relationship between the dipole moment of the methylammonium cation and the optoelectronic properties of lead halide perovskites remains under debate. We show that both the temperature-dependent charge carrier mobility and recombination kinetics are identical for methylammonium and cesium lead iodide, indicating that the role of the...
journal article 2018
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Bartesaghi, D. (author), Ray, Aniruddha (author), Jiang, Junke (author), Bouwer, Ricardo K.M. (author), Tao, S. (author), Savenije, T.J. (author)
Tailoring the physical properties of hybrid lead metal halide APbX<sub>3</sub> perovskites by means of compositional engineering is one of the key factors contributing to the development of highly efficient and stable perovskite solar cells. While the beneficial effects of partial ionic replacement at the A- and X-sites are largely...
journal article 2018
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Bartesaghi, D. (author), Slavney, Adam H. (author), Gelvez Rueda, M.C. (author), Connor, Bridget A. (author), Grozema, F.C. (author), Karunadasa, Hemamala I. (author), Savenije, T.J. (author)
Double perovskites, comprising two different cations, are potential nontoxic alternatives to lead halide perovskites. Here, we characterized thin films and crystals of Cs<sub>2</sub>AgBiBr<sub>6</sub> by time-resolved microwave conductance (TRMC), which probes formation and decay of mobile charges upon pulsed irradiation. Optical excitation...
journal article 2018
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Maheswari, S. (author), Savenije, T.J. (author), Renaud, N. (author), Grozema, F.C. (author)
Two-dimensional (2D) halide perovskites are a class of materials in which 2D layers of perovskite are separated by large organic cations. Conventionally, the 2D perovskites incorporate organic cations as spacers, but these organic cations also offer a route to introduce specific functionality in the material. In this work, we demonstrate, by...
journal article 2018
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Gelvez Rueda, M.C. (author), Hutter, E.M. (author), Cao, Duyen H. (author), Renaud, N. (author), Stoumpos, Constantinos C. (author), Hupp, Joseph T. (author), Savenije, T.J. (author), Kanatzidis, Mercouri G. (author), Grozema, F.C. (author)
The optoelectronic properties of hybrid perovskites can be easily tailored by varying their components. Specifically, mixing the common short organic cation (methylammonium (MA)) with a larger one (e.g., butyl ammonium (BA)) results in 2-dimensional perovskites with varying thicknesses of inorganic layers separated by the large organic cation...
journal article 2017
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Guo, Dengyang (author), Bartesaghi, D. (author), Wei, Haotong (author), Hutter, E.M. (author), Huang, Jinsong (author), Savenije, T.J. (author)
In view of its band gap of 2.2 eV and its stability, methylammonium lead bromide (MAPbBr<sub>3</sub>) is a possible candidate to serve as a light absorber in a subcell of a multijunction solar cell. Using complementary temperature-dependent time-resolved microwave conductance (TRMC) and photoluminescence (TRPL) measurements, we demonstrate...
journal article 2017
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