Searched for: author%3A%22van+Ommen%2C+J.R.%22
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Graas, Adriaan B.M. (author), Wagner, E.C. (author), van Leeuwen, Tristan (author), van Ommen, J.R. (author), Batenburg, K. Joost (author), Lucka, Felix (author), Portela, L. (author)
A new X-ray computed tomography technique for the purpose of imaging fluidized beds is presented. It consists of an experimental set-up with three stationary X-ray source and flat panel detector pairs, a geometric calibration and data processing workflow, and an image reconstruction algorithm. The technique enables sparse-angular tomographic...
journal article 2024
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Bleeker, J.J. (author), van Kasteren, Celine (author), van Ommen, J.R. (author), Vermaas, D.A. (author)
To make green hydrogen more economically attractive, the energy losses in alkaline electrolysis need to be minimized while operating at high current densities (1 A cm<sup>−2</sup>). At these current densities the ohmic resistance and gas bubbles effects contribute largely to the energy losses. To mitigate the gas bubbles losses, we...
journal article 2024
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Kamphorst, R. (author), Wanjari, Pratyush (author), Saedy, S. (author), van Dam, Julia F.K. (author), Thijssen, A. (author), Brüner, Philipp (author), Grehl, Thomas (author), Meesters, G.M.H. (author), van Ommen, J.R. (author)
In this study, we investigated the wettability and agglomeration characteristics of polymer microspheres coated with low-temperature deposited SiO<sub>2</sub> in a fluidized bed atomic layer deposition (ALD) setup. Surface characterization revealed the presence of a significant amount of deposited Si-OH groups within the first cycles. A...
journal article 2024
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Kamphorst, R. (author), van der Sande, P.C. (author), Wu, K. (author), Wagner, E.C. (author), David, M.K. (author), Meesters, G.M.H. (author), van Ommen, J.R. (author)
Vibro-assisted fluidization of cohesive micro-silica has been studied by means of X-ray imaging, pressure drop measurements, and off-line determination of the agglomerate size. Pressure drop and bed height development could be explained by observable phenomena taking place in the bed; slugging, channeling, fluidization or densification. It...
journal article 2024
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van der Sande, P.C. (author), Wagner, E.C. (author), de Mooij, Jack (author), Meesters, G.M.H. (author), van Ommen, J.R. (author)
Horizontal stirred bed reactors are widely used in the commercial manufacturing of polypropylene. However, a comprehensive understanding of the particle dynamics in horizontal stirred bed reactors remains elusive, primarily due to the lack of detailed experimental data. In this work, we studied the influence of operating parameters on the...
journal article 2024
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Li, M. (author), Saedy, S. (author), Fu, S. (author), Stellema, T.P. (author), Kortlever, R. (author), van Ommen, J.R. (author)
Extending the lifetime of electrocatalytic materials is a major challenge in electrocatalysis. Here, we employ atomic layer deposition (ALD) to coat the surface of carbon black supported platinum nanoparticles (Pt/CB) with an ultra-thin layer of silicon dioxide (SiO2) to prevent deactivation of the catalyst during H2 evolution. Our results show...
journal article 2024
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Kamphorst, R. (author), Wu, K. (author), van Baarlen, M. (author), Meesters, G.M.H. (author), van Ommen, J.R. (author)
In this study, the impact of different vibrational modes on the fluidization characteristics of cohesive micro- and nano-silica powder was examined. Fractional pressure drop, bed expansion measurements, and X-ray imaging were utilized to characterize the fluidization quality. The densities of the emulsion phase at the top and bottom of the...
journal article 2024
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Wu, K. (author), Kamphorst, R. (author), Bakker, A.M.T. (author), Ford, Jasper (author), Wagner, E.C. (author), Ochkin-Koenig, Olga (author), Franck, Miika (author), Weis, Dominik (author), Meesters, G.M.H. (author), van Ommen, J.R. (author)
Stirring has been recognized in the literature as a promising technique for facilitating fluidization of cohesive powders, via inputting additional energy to counteract interparticle forces. However, the influence of operating conditions and stirrer configurations on flow behavior remains largely unknown, which impedes the practical...
journal article 2024
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Wu, Y. (author), Liu, Daoyin (author), van Wachem, Berend G.M. (author), van Ommen, J.R. (author)
Nanoparticles are usually fluidized as agglomerates, which are in dynamic states of agglomeration and fragmentation. It is critical to consider the size distribution of agglomerates in modeling of the fluidization of nanoparticle agglomerates. In this article, the fluidization behavior of nanoparticle agglomerates is investigated using a two...
journal article 2024
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Sajeev Kumar, A. (author), Moura de Salles Pupo, M. (author), Petrov, K.V. (author), Ramdin, M. (author), van Ommen, J.R. (author), de Jong, W. (author), Kortlever, R. (author)
Aqueous electrolytes used in CO2 electroreduction typically have a CO2 solubility of around 34 mM under ambient conditions, contributing to mass transfer limitations in the system. Non-aqueous electrolytes exhibit higher CO2 solubility (by 5–8-fold) and also provide possibilities to suppress the undesired hydrogen evolution reaction (HER). On...
journal article 2023
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Moulijn, J.A. (author), van Ommen, J.R. (author), Goulas, A. (author), Valdesueiro Gonzalez, D. (author), Juan-Alcañiz, Jana (author), Au-Yeung, Kar Ming (author), Woning, Leo (author), Bergwerff, Jaap A. (author)
The feasibility of gas phase deposition using a Ti alkoxide precursor for precise surface modification of catalysts was demonstrated by modifying a mesoporous alumina support with a Ti oxide overcoat. Titanium tetra-isopropoxide yields a Ti oxide layer that covers homogeneously the alumina surface. Uniformity of the deposited TiO<sub>2</sub>...
journal article 2023
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Zhao, Y. (author), Wang, Xiao (author), Li, Quan an (author), Zhang, Xinyu (author), Li, Ye (author), Xie, Rong Jun (author), van Ommen, J.R. (author), Hintzen, H.T.J.M. (author)
The cyan-emitting BaSi<sub>2</sub>O<sub>2</sub>N<sub>2</sub>:Eu<sup>2+</sup> phosphor is a promising narrow-band and high-efficiency luminescent material used in wide-color-gamut white light-emitting diodes (wLEDs). However, its serious degradation under thermal attacks hinders its practical applications and needs to be improved. Herein, we...
journal article 2023
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Mahtabani, Amirhossein (author), La Zara, D. (author), Niittymäki, Minna (author), Anyszka, Rafał (author), Rytöluoto, Ilkka (author), He, Xiaozhen (author), Saarimäki, Eetta (author), Saedy, S. (author), van Ommen, J.R. (author)
Polymer nanocomposites (NCs) offer outstanding potential for dielectric applications including insulation materials. The large interfacial area introduced by the nanoscale fillers plays a major role in improving the dielectric properties of NCs. Therefore, an effort to tailor the properties of these interfaces can lead to substantial...
journal article 2023
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Wu, K. (author), Wagner, E.C. (author), Ochkin-Koenig, Olga (author), Franck, Miika (author), Weis, Dominik (author), Meesters, G.M.H. (author), van Ommen, J.R. (author)
Mechanical vibration has been broadly used to assist fluidization of cohesive powders, because of its capability to disrupt gas channels and agglomerates. However, the improvement reported in literature is mostly deduced from bulk response and ex-situ measurements, whereas the induced fluidization behavior and underlying physics remain...
journal article 2023
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Nederstigt, Tom A.P. (author), Bode, Bo (author), van Ommen, J.R. (author), Peijnenburg, Willie J.G.M. (author), Vijver, Martina G. (author)
Novel nanomaterial-based pesticide formulations are increasingly perceived as promising aids in the transition to more efficient agricultural production systems. The current understanding of potential unintended (eco)toxicological impacts of nano-formulated pesticides is scarce, in particular with regard to (non-target) aquatic organisms and...
journal article 2023
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Bagemihl, I. (author), Cammann, Lucas (author), Pérez-Fortes, Mar (author), van Steijn, V. (author), van Ommen, J.R. (author)
The production of base chemicals by electrochemical conversion of captured CO<sub>2</sub> has the potential to close the carbon cycle, thereby contributing to a future energy transition. With the feasibility of low-temperature electrochemical CO<sub>2</sub> conversion demonstrated at lab scale, research is shifting toward optimizing...
journal article 2023
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Kim, S. (author), Dierkes, Wilma K. (author), Blume, Anke (author), Talma, Auke (author), van Ommen, J.R. (author), Courtois, Nicolas (author), Davin, Julian (author), Recker, Carla (author), Schoeffel, Julia (author)
Pre-treated silica with a plasma-deposited (PD) layer of polymerized precursors was tested concerning its compatibility with Natural Rubber (NR) and its influence on the processing of silica-silane compounds. The modification was performed in a tailor-made plasma reactor. The degree of deposition of the plasma-coated samples was analyzed by...
journal article 2023
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Uglietti, R. (author), Micale, Daniele (author), La Zara, D. (author), Goulas, A. (author), Nardi, Luca (author), Bracconi, Mauro (author), van Ommen, J.R. (author), Maestri, Matteo (author)
We show the potential of coupling numerical and experimental approaches in the fundamental understanding of catalytic reactors, and in particular fluidized beds. The applicability of the method was demonstrated in a lab-scale fluidized bed reactor for the platinum-based catalytic oxidation of hydrogen. An experimental campaign has been...
journal article 2023
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Zhang, F. (author), Wu, K. (author), La Zara, D. (author), Sun, F. (author), Quayle, Michael J. (author), Petersson, Gunilla (author), Folestad, Staffan (author), Chew, Jia Wei (author), van Ommen, J.R. (author)
For dry powder inhaled formulations, good flow behaviour is vital in re-dispersing the powder. However, inhaled drug powders with a particle size below 10 µm are classified as highly cohesive materials with poor flow characteristics. Here we demonstrate how to alter the flow properties of micronized budesonide powders by depositing different...
journal article 2023
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Santoso, A. (author), Damen, Afke (author), van Ommen, J.R. (author), van Steijn, V. (author)
We explore three variants of atomic layer deposition (ALD) to deposit titanium oxide on the soft polymer polydimethylsiloxane (PDMS). We show that the organic solvent resistance of PDMS is increased by two orders of magnitude compared to uncoated PDMS for ALD performed at atmospheric pressure, which results in a unique surface-subsurface...
journal article 2022
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