Searched for: subject%3A%22Water%25E2%2580%2593gas%255C+shift%255C+reaction%22
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Ariëns, M.I. (author), van de Water, L. G.A. (author), Dugulan, A.I. (author), Brück, E.H. (author), Hensen, E. J.M. (author)
Copper promotion of chromium-doped iron oxide prepared via co-precipitation for high-temperature water–gas shift (WGS) catalysis is investigated. Low-temperature Mössbauer spectra demonstrate that copper doping delays hematite (α-Fe<sub>2</sub>O<sub>3</sub>) formation in the fresh catalyst, favoring the formation of small crystallites of...
journal article 2022
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Ariëns, M.I. (author), Van De Water, L. G.A. (author), Dugulan, A.I. (author), Brück, E.H. (author), Hensen, E. J.M. (author)
A set of doped iron oxides (chromium, aluminum, gallium, indium, manganese, zinc, niobium) were prepared by a one-step coprecipitation/calcination approach evaluated for their WGS activity under industrially relevant conditions and characterized in detail. The WGS activity after ageing the doped catalyst for 4 days at 25 bar follows the order...
journal article 2022
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Cavalli, A. (author), Chundru, P. (author), Brunner, Thomas (author), Obernberger, Ingwald (author), Mirabelli, Ilaria (author), Makkus, Robert (author), Aravind, P.V. (author)
High temperature biosyngas cleaning is more efficient when the end user operates at elevated temperature, as in biomass gasifier solid oxide fuel cell systems. However, there is not much experience with this technology and low temperature gas cleaning is usually adopted. This paper advances current knowledge by presenting the results from the...
journal article 2021
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Ariëns, M.I. (author), Chlan, V. (author), Novák, P. (author), van de Water, L. G.A. (author), Dugulan, A.I. (author), Brück, E.H. (author), Hensen, E. J.M. (author)
Chromium promotion of iron oxide based water-gas shift (WGS) catalysts prepared via co-precipitation/calcination was investigated. Mössbauer spectroscopy and XRD evidence that chromium is incorporated in the calcined hematite (α-Fe<sub>2</sub>O<sub>3</sub>) precursor irrespective of the doping level (0−12 wt.%). CO-TPR shows chromium delays...
journal article 2021
Searched for: subject%3A%22Water%25E2%2580%2593gas%255C+shift%255C+reaction%22
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