A Novel Multiple-Ring Aromatic Spacer Based 2D Ruddlesden–Popper CsPbI₃ Solar Cell with Record Efficiency Beyond 16%

Two-dimensional (2D) Ruddlesden–Popper (RP) CsPbI₃ perovskite possesses superior phase stability by introducing steric hindrance. However, due to the quantum and dielectric confinement effect, 2D structures usually exhibit large exciton binding energy, and the charge tunneling barrier across the organic interlayer is difficult to...