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Lead emissions from road transport in Europe. A revision of current estimates using various estimation methodologies

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Author: Denier van der Gon, H.A.C. · Appelman, W.
Type:article
Date:2009
Institution: TNO Bouw en Ondergrond
Source:Science of the Total Environment, 20, 407, 5367-5372
Identifier: 241776
Keywords: Environment · Air pollution · Emission inventories · Fuel quality · Lead · Road transport · Atmospheric lead · Current estimates · Emission estimation methodologies · Emission inventories · Estimation methodologies · Exhaust emission · Fuel quality · Fuel samples · Lead additives · Lead concentration · Lead content · Lead emission · Leaded gasoline · Model-predicted concentrations · Road transport · Road transports · Total emissions · Unleaded gasoline · Air quality · Atmospheric chemistry · Atmospheric movements · Combustion · Concentration (process) · Fuels · Gasoline · Laws and legislation · Motor transportation · Roads and streets · Thermochemistry · Uncertainty analysis · Lead · gasoline · lead · air quality · atmospheric pollution · combustion · concentration (composition) · estimation method · lead · pollutant source · road transport · traffic emission · air pollution · article · atmospheric dispersion · chemical analysis · combustion · concentration process · environmental monitoring · Europe · exhaust gas · priority journal · uncertainty · Eurasia · Europe

Abstract

Large-scale use of leaded gasoline was an important source of the neurotoxin lead in the European environment. After a sequence of regulations on the allowed gasoline lead content and, eventually, a ban on the use of lead additives in gasoline, road transport was no longer considered a source of atmospheric lead. Currently a discrepancy exists between measured atmospheric lead concentrations and model-predicted concentrations, suggesting that lead emissions to the atmosphere may be underestimated. Recently it was suggested that lead emission from unleaded gasoline combustion is still an important source and may (partly) fill the gap between modelled and observed atmospheric lead concentrations. In this paper we assess the plausibility of the latter suggestion by following various emission estimation methodologies. The uncertainty of lead emissions from road transport is further reduced by chemical analysis of fuel samples. The result of our assessment is that lead from road transport fuel combustion is not the missing lead source needed to fill the gap between modelled and observed lead concentrations. Road transport is still a source of lead through brake wear and a small contribution from exhaust emissions but this contributes no more than 5-8% of the EU25 total emission. © 2009 Elsevier B.V. All rights reserved.