Dynamic Polymer Hydrogels through Reversible Thiol Conjugate Addition Crosslinks

This thesis describes the experimental development of new dynamic hydrogels based on reversible thiol conjugate additions. Redox-controlled hydrogels and self-healing injectable hydrogels have been achieved by introducing reversible thiol conjugate additions to crosslink polymers, leading to hydrogel formation. The overall objective in this...

Structure and Dynamics of Self-Healing Polyurethanes

The work exposed in this thesis addresses two main scientific challenges in the field of intrinsic self-healing polymers that limit the translation of the academic research efforts into commercial products, namely: i) the implementation of the self-healing functionality in polymer commodities by minimal chemical modifications; and ii) the...