A triad of high-field magnetic transitions in V5S8
C. A. Sonego (Federal University of ABC, University of Cambridge, Cavendish Laboratory)
P. M.T. Vianez (Cavendish Laboratory, University of Cambridge)
H. Li (Cavendish Laboratory, University of Cambridge)
J. C. Lashley (Cavendish Laboratory, University of Cambridge)
G. G. Lonzarich (University of Cambridge, Cavendish Laboratory)
M. N. Ali (TU Delft - QN/Ali Lab, Kavli institute of nanoscience Delft)
M. A. Avila (Federal University of ABC)
S. E. Rowley (University of Cambridge, Cavendish Laboratory)
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Abstract
We report the observation of an unexpected phase transition at high magnetic fields between the spin-flop and spin-flip transitions in the d-electron antiferromagnetic metal V5S8. High-precision magnetic, thermal and electrical transport measurements enable the transitions to be tracked up to fields as high as 35 T and at temperatures down to the milli-kelvin range revealing three distinct magnetic quantum phase transitions. We present a model that finds agreement with our observation of a triad of spin transitions involving two sublattices with frustrated inter-and intra-sublattice spin couplings.