Model-based optimization of a photocatalytic reactor with light-emitting diodes

Journal Article (2016)
Author(s)

Fatemeh Khodadadian (TU Delft - Mechanical Engineering)

Ali Poursaeidesfahani (TU Delft - Mechanical Engineering)

Zonghan Li

J. Ruud van Ommen (TU Delft - Applied Sciences)

Andrzej I. Stankiewicz (TU Delft - Mechanical Engineering)

Richard Lakerveld (The Hong Kong University of Science and Technology)

Research Group
Intensified Reaction and Separation Systems
DOI related publication
https://doi.org/10.1002/ceat.201600010 Final published version
More Info
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Publication Year
2016
Language
English
Research Group
Intensified Reaction and Separation Systems
Issue number
10
Volume number
39
Pages (from-to)
1946-1954
Downloads counter
151

Abstract

The complicated interplay between mass and photon transfer within a photocatalytic reactor calls for an integrated design approach. A model-based optimization approach for LED-based photocatalytic reactors is presented. First, a model that describes the distribution of reactants and photons within a photocatalytic reactor is developed. Then, several design variables related to the reactor dimensions and light sources are optimized simultaneously using the photocatalytic degradation of toluene as a model system. The results demonstrate how different formulations of the problem can be used to either minimize the reactor cost or to obtain a specified concentration profile within the reactor.