In situ study of electric field controlled ion transport in the Fe/BaTiO3 interface
D. G. Merkel (European Synchrotron Radiation Facility, Hungarian Academy of Sciences)
D. Bessas (TU Delft - Applied Sciences, European Synchrotron Radiation Facility)
G. Bazsó (Hungarian Academy of Sciences)
A. Jafari (Technical University of Denmark (DTU), European Synchrotron Radiation Facility)
R. Rüffer (European Synchrotron Radiation Facility)
A. I. Chumakov (European Synchrotron Radiation Facility)
N. Q. Khanh (Institute of Technical Physics and Materials Science)
Sz Sajti (Hungarian Academy of Sciences)
J. P. Celse (European Synchrotron Radiation Facility)
D. L. Nagy (Hungarian Academy of Sciences)
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Abstract
Electric field controlled ion transport and interface formation of iron thin films on a BaTiO3 substrate have been investigated by in situ nuclear resonance scattering and x-ray reflectometry techniques. At early stage of deposition, an iron-II oxide interface layer was observed. The hyperfine parameters of the interface layer were found insensitive to the evaporated layer thickness. When an electric field was applied during growth, a 10 Å increase of the nonmagnetic/magnetic thickness threshold and an extended magnetic transition region was measured compared to the case where no field was applied. The interface layer was found stable under this threshold when further evaporation occurred, contrary to the magnetic layer where the magnitude and orientation of the hyperfine magnetic field vary continuously. The obtained results of the growth mechanism and of the electric field effect of the Fe/BTO system will allow the design of novel applications by creating custom oxide/metallic nanopatterns using laterally inhomogeneous electric fields during sample preparation.