Methane dehydroaromatization catalyzed by Mo/ZSM-5
location-steered activity and mechanism
G. Li (Wageningen University & Research, TU Delft - ChemE/Inorganic Systems Engineering)
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Abstract
This work examined the location-steered catalytic behavior of Mo/ZSM-5 catalyst for one-step methane dehydroaromatization to benzene reaction. The results indicated that α-site is the preferred location for the formation of ethylene, the main intermediate for aromatics production via the propagation pathway, while δ-site is favorable for the hydrocarbon pool aggregation reaction pathway.
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