Corrosion protection in a coating defect on AA2024-T3 by lithium carbonate inhibitor leaching

An experimentally validated FEM approach

Journal Article (2025)
Author(s)

N. Abdelrahman (Vrije Universiteit Brussel)

N. Van den Steen (Vrije Universiteit Brussel)

C. Özkan (TU Delft - Team Arjan Mol)

P. Visser (Akzo Nobel)

S. V. Lamaka (Helmholtz-Zentrum Hereon)

R. Böttcher (Airbus)

J. M.C. Mol (TU Delft - Team Arjan Mol)

H. Terryn (Vrije Universiteit Brussel, TU Delft - Team Arjan Mol)

T. Hauffman (Vrije Universiteit Brussel)

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Research Group
Team Arjan Mol
DOI related publication
https://doi.org/10.1016/j.corsci.2025.112861
More Info
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Publication Year
2025
Language
English
Research Group
Team Arjan Mol
Bibliographical Note
Green Open Access added to TU Delft Institutional Repository 'You share, we take care!' - Taverne project https://www.openaccess.nl/en/you-share-we-take-care Otherwise as indicated in the copyright section: the publisher is the copyright holder of this work and the author uses the Dutch legislation to make this work public.
Journal title
Corrosion Science
Volume number
250
Article number
112861
Downloads counter
291
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Abstract

A 2D finite element model is developed to simulate the protection of active protective coatings in a defect. The leaching kinetics, inhibitor-electrolyte reactions and electrochemical surface reactions on homogenized AA2024-T3, are considered. Changes in local oxygen distribution, pH, and current density over time are validated using surface scanning micro-probe techniques. The limitations posed by the prediction of surface current density at the metal interface using a FEM model with a homogenized microstructure are identified and addressed. The validated FEM is then used to predict inhibitor concentration and pH dependent on the initial inhibitor pigment concentration in an organic coating.

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