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Lin, P. (author), Liu, X. (author), Ren, S. (author), Li, Yi (author), Erkens, S. (author), Welvaarts, B. (author), Brouns, K. (author)Developed by Delft University of Technology, the tri-component polyurethane modified cold binder (PMCB) displays impressive durability and strength in asphalt mixtures, showing promise as a reliable binder for cold in-place recycling. However, when applying PMCB for rapid, in-situ recycling, the presence of moisture in reclaimed asphalt...conference paper 2024
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Assaf Martinez-Streignard, E.I. (author), Liu, X. (author), Lin, P. (author), Erkens, S. (author)This paper presents a United Atom (UA) force field for simulating hydrocarbon molecules in bituminous materials, integrating explicit hydrogens into beads with their parent atom. This method simplifies all-atom molecular models, significantly accelerating Molecular Dynamics (MD) simulations of bitumen by 10 to 100 times. Key advantages...journal article 2024
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Lin, P. (author), Liu, X. (author), Erkens, S. (author), Welvaarts, Bart (author), Brouns, Koen (author)Cold in-place recycling is gaining more attention worldwide because of its lower energy consumption, while the normally used asphalt emulsion and foamed asphalt cannot meet this requirement of short traffic disturbance and road performance of the surface layer. In this research, a polyurethane-modified cold binder (PMCB) was designed and...journal article 2023
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Assaf Martinez-Streignard, E.I. (author), Liu, X. (author), Lin, P. (author), Erkens, S. (author), Nahar, Sayeda (author), Mensink, Liz I.S. (author)Conventional Molecular Dynamics (MD) models of bitumen are built by homogeneously mixing molecules in a volume without considering that the molecules in bitumen are known to exhibit phase behavior and form distinctive molecular arrangements. These are known to have a significant impact in the behavior of bitumen, and considering their...journal article 2023
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Ren, S. (author), Liu, X. (author), Jing, R. (author), Gao, Y. (author), Lin, P. (author), Erkens, S. (author)Two types of elastomer/plastic compound-modified bitumen were developed by means of incorporating the reactive elastomeric terpolymer (RET) into the plastic (high-density polyethylene HDPE or recycled polyethylene RPE) modified bitumen and adding the wax residue (WR) into the bitumen/elastomer (crumb rubber CR or styrene–butadiene–styrene SBS)...journal article 2023
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Ren, S. (author), Liu, X. (author), Gao, Y. (author), Jing, R. (author), Lin, P. (author), Erkens, S. (author), Wang, H. (author)This study aims to multiscale investigate the effects of rejuvenator type, temperature, and aging degree of bitumen on the diffusion behaviors of rejuvenators (bio-oil BO, engine-oil EO, naphthenic-oil NO, and aromatic-oil AO) in aged binders. The molecular dynamics (MD) simulation method is performed to detect the molecular-level diffusion...journal article 2023
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Ren, S. (author), Liu, X. (author), van Aggelen, M. (author), Lin, P. (author), Erkens, S. (author)This study investigates the impacts of rejuvenator type/dosage and the aging degree of bitumen on the chemical and rheological properties of rejuvenated bitumen, and propose critical chemo-rheological indicators for evaluating rejuvenation efficiency. Moreover, the potential connections between essential chemical and rheological indices of...journal article 2023
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Ren, S. (author), Liu, X. (author), Lin, P. (author), Gao, Y. (author), Erkens, S. (author)Molecular dynamics (MD) simulation plays an effective role in predicting the critical properties and explaining the macroscale phenomenon at the nanoscale. This review summarized the application cases of MD simulations in various bitumen systems, considering aging, modification, and rejuvenation factors. Meanwhile, the potential relationships...review 2022
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Ren, S. (author), Liu, X. (author), Lin, P. (author), Gao, Y. (author), Erkens, S. (author)The cohesive and adhesive performances of bituminous materials significantly affect the service life of asphalt pavement. The molecular dynamics (MD) simulation method has been proved as an effective tool to predict the thermodynamics parameters of different multisubstance and multi-phase bitumen models during different diffusion, self-healing,...review 2022
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Zhang, Y. (author), Liu, X. (author), Ren, S. (author), Jing, R. (author), Lin, P. (author), Apostolidis, P. (author), Erkens, S. (author), Wang, Xuancang (author), Scarpas, Athanasios (author)Lignin, one of the most abundant natural polymers, has been extensively studied as an additive in bituminous binders. Even though the lignin improves the overall resistance against oxidative aging of bitumen, it could lead to high thermal cracking sensitivity. In this study, a bio-oil (i.e., rapeseed oil) is implemented in lignin-modified...journal article 2022
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Ren, S. (author), Liu, X. (author), Lin, P. (author), Gao, Y. (author), Erkens, S. (author)The compatibility potential of rejuvenators plays an important role in improving the blending degree of rejuvenated bitumen. This study aims at estimating the efficiency of molecular dynamics (MD) simulation in predicting the compatibility between rejuvenators and aged bitumen, and exploring the influence of rejuvenator type, aging degree of...journal article 2022
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Ren, S. (author), Liu, X. (author), Lin, P. (author), Erkens, S. (author)This study investigated the effects of swelling-degradation degree on the rheological properties and thermal pyrolysis behaviors of crumb rubber modified bitumen (CRMB). The equilibrium viscosity of CRMB in 160 ◦Cswelling process is 10.5 Pa·s at 8 h. During the 200℃-degradation procedure, the viscosity increased to a maximum value of 20.58 Pa·s...journal article 2022
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Ren, S. (author), Liu, X. (author), Erkens, S. (author), Lin, P. (author), Gao, Y. (author)The molecular dynamics (MD) simulation method is proved as an efficient tool to explore the intermolecular interaction between rejuvenators and aged bitumen, but the simple “singlemolecule” model of rejuvenator would bring the inaccuracy to simulation outputs due to a huge difference with its realistic multi-component chrematistic. This study...journal article 2022
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Ren, S. (author), Liu, X. (author), Lin, P. (author), Jing, R. (author), Erkens, S. (author)This study aimed to explore the long-term aging influence on chemo rheological properties and develop novel consecutive models for the long-term aging reaction kinetics of bitumen. The results revealed that the aging index was significantly dependent on the types of selected parameters. The Zero-order model was suitable to describe the long-term...journal article 2022
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Ren, S. (author), Liu, X. (author), Lin, P. (author), Erkens, S. (author), Gao, Y. (author)Molecular dynamics (MD) simulation is an advanced tool to explore the interaction mechanism between aged bitumen and rejuvenators at the nanoscale. However, the general MD molecular structures of rejuvenators led to the lower quantify and inaccuracy of the simulation outputs. This study aims at developing more realistic molecular models to...journal article 2022
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Ren, S. (author), Liu, X. (author), Lin, P. (author), Erkens, S. (author), Xiao, Yue (author)To further explore the long-term aging behaviors of bitumen from the multiscale perspectives, the experimental characterization and molecular dynamics (MD) simulation methods were performed. Series of chemical properties for the virgin and various aged bitumen were evaluated using the TCL-FID, ATR-FTIR, Elemental analysis and GPC tests. The...journal article 2021
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Ren, S. (author), Liu, X. (author), Lin, P. (author), Wang, H. (author), Fan, W. (author), Erkens, S. (author)The chemo-rheological properties of crumb rubber modified bitumen are always unstable due to the mutable and uncontrollable swelling-degradation degree of crumb rubber in bitumen matrix. The study aimed at exploring the continuous swelling and degradation behaviors of crumb rubber modified bitumen (CRMB) considering the influence of rubber size...journal article 2021
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Ren, S. (author), Liu, X. (author), Lin, P. (author), Erkens, S. (author)This study elaborates the influence of blends formulated by waste oil (WO) and styrene-butadiene rubber (SBR) on thermo-mechanical and chemical compositional characteristics of rejuvenated bitumen. The results show that both WEO (waste engine oil) and WCO (waste cooking oil) can compensate viscous component for reclaimed bitumen, and the effect...conference paper 2021
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Lin, P. (author), Liu, X. (author), Apostolidis, P. (author), Erkens, S. (author), Zhang, Y. (author), Ren, S. (author)Observing the microstructure of bituminous binders with an environmental scanning electron microscope (ESEM) can contribute significantly to reveal the underlying rejuvenation mechanism. In this study, three rejuvenators were selected to regenerate the aged SBS modified binders at five dosages, and their rheology was evaluated using a dynamic...journal article 2021
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Ren, S. (author), Liu, X. (author), Zhang, Y. (author), Lin, P. (author), Apostolidis, P. (author), Erkens, S. (author), Li, Mingliang (author), Xu, Jian (author)Lignin, as a major waste from biofuel and paper industries, could be utilized as a modifier to enhance the relevant performance of bitumen. However, the effects of lignin on the thermodynamics properties and molecular structure of bitumen are rarely studied. Meanwhile, the potential modification mechanism of lignin modified bitumen is still...journal article 2021