Investigating the impact of coupling HARMONIE-WINS50 (cy43) meteorology to LOTOS-EUROS (v2.2.002) on a simulation of NO2 concentrations over the Netherlands

Meteorological fields calculated by numerical weather prediction (NWP) models drive offline chemical transport models (CTMs) to solve the transport, chemical reactions, and atmospheric interaction over the geographical domain of interest. HARMONIE (HIRLAM ALADIN Research on Mesoscale Operational NWP in Euromed) is a state-of-The-Art non...

A gridded air quality forecast through fusing site-available machine learning predictions from RFSML v1.0 and chemical transport model results from GEOS-Chem v13.1.0 using the ensemble Kalman filter

Statistical methods, particularly machine learning models, have gained significant popularity in air quality predictions. These prediction models are commonly trained using the historical measurement datasets independently collected at the environmental monitoring stations and their operational forecasts in advance using inputs of the real-time...

Advecting Superspecies: Efficiently Modeling Transport of Organic Aerosol With a Mass-Conserving Dimensionality Reduction Method

The chemical transport model LOTOS-EUROS uses a volatility basis set (VBS) approach to represent the formation of secondary organic aerosol (SOA) in the atmosphere. Inclusion of the VBS approximately doubles the dimensionality of LOTOS-EUROS and slows computation of the advection operator by a factor of two. This complexity limits SOA...

Improving Air Pollution Modelling in Complex Terrain with a Coupled WRF–LOTOS–EUROS Approach: A Case Study in Aburrá Valley, Colombia

Chemical transport models (CTM) are crucial for simulating the distribution of air pollutants, such as particulate matter, and evaluating their impact on the environment and human health. However, these models rely heavily on accurate emission inventory and meteorological inputs, usually obtained from reanalyzed weather data, such as the...

Dust storm forecasting through coupling LOTOS-EUROS with localized ensemble Kalman filter

Super dust storms re-occurred over East Asia in 2021 spring and casted great health damages and property losses. It is essential to achieve an accurate dust forecast to reduce the damage for early warning. The forecasting system fundamentally relies on a numerical model which can forecast the full evolution of dust storms. However, large...

Development of a regional feature selection-based machine learning system (RFSML v1.0) for air pollution forecasting over China

With the explosive growth of atmospheric data, machine learning models have achieved great success in air pollution forecasting because of their higher computational efficiency than the traditional chemical transport models. However, in previous studies, new prediction algorithms have only been tested at stations or in a small region; a large...

A Knowledge-Aided Robust Ensemble Kalman Filter Algorithm for Non-Linear and Non-Gaussian Large Systems

This work proposes a robust and non-Gaussian version of the shrinkage-based knowledge-aided EnKF implementation called Ensemble Time Local H_∞ Filter Knowledge-Aided (EnTLHF-KA). The EnTLHF-KA requires a target covariance matrix to integrate previously obtained information and knowledge directly into the data assimilation (DA). The...

Inverse modeling of the 2021 spring super dust storms in East Asia

Last spring, super dust storms reappeared in East Asia after being absent for one and a half decades. The event caused enormous losses in both Mongolia and China. Accurate simulation of such super sandstorms is valuable for the quantification of health damage, aviation risks, and profound impacts on the Earth system, but also to reveal the...

Estimating NOx LOTOS-EUROS CTM Emission Parameters over the Northwest of South America through 4DEnVar TROPOMI NO2 Assimilation

In this work, we present the development of a 4D-Ensemble-Variational (4DEnVar) data assimilation technique to estimate NOx top-down emissions using the regional chemical transport model LOTOS-EUROS with the NO2 observations from the TROPOspheric Monitoring Instrument (TROPOMI). The assimilation was performed for a domain in the northwest of...

Urban air quality modeling using low-cost sensor network and data assimilation in the aburrá valley, colombia

The use of low air quality networks has been increasing in recent years to study urban pollution dynamics. Here we show the evaluation of the operational Aburrá Valley’s low-cost network against the official monitoring network. The results show that the PM_2.5 low-cost measurements are very close to those observed by the official...

Position correction in dust storm forecasting using LOTOS-EUROS v2.1: Grid-distorted data assimilation v1.0

When calibrating simulations of dust clouds, both the intensity and the position are important. Intensity errors arise mainly from uncertain emission and sedimentation strengths, while position errors are attributed either to imperfect emission timing or to uncertainties in the transport. Though many studies have been conducted on the...

An efficient ensemble Kalman Filter implementation via shrinkage covariance matrix estimation: exploiting prior knowledge

In this paper, we propose an efficient and practical implementation of the ensemble Kalman filter via shrinkage covariance matrix estimation. Our filter implementation combines information brought by an ensemble of model realizations, and that based on our prior knowledge about the dynamical system of interest. We perform the combination of...

Source backtracking for dust storm emission inversion using an adjoint method: Case study of Northeast China

Emission inversion using data assimilation fundamentally relies on having the correct assumptions about the emission background error covariance. A perfect covariance accounts for the uncertainty based on prior knowledge and is able to explain differences between model simulations and observations. In practice, emission uncertainties are...

Machine learning for observation bias correction with application to dust storm data assimilation

Data assimilation algorithms rely on a basic assumption of an unbiased observation error. However, the presence of inconsistent measurements with nontrivial biases or inseparable baselines is unavoidable in practice. Assimilation analysis might diverge from reality since the data assimilation itself cannot distinguish whether the differences...

Dust Emission Inversion Using Himawari-8 AODs Over East Asia: An Extreme Dust Event in May 2017

Aerosol optical depths (AODs) from the new Himawari-8 satellite instrument have been assimilated in a dust simulation model over East Asia. This advanced geostationary instrument is capable of monitoring the East Asian dust storms which usually have great spatial and temporal variability. The quality of the data has been verified through a...

Accelerating volcanic ash data assimilation using a mask-state algorithm based on an ensemble Kalman filter: A case study with the LOTOS-EUROS model (version 1.10)

In this study, we investigate a strategy to accelerate the data assimilation (DA) algorithm. Based on evaluations of the computational time, the analysis step of the assimilation turns out to be the most expensive part. After a study of the characteristics of the ensemble ash state, we propose a mask-state algorithm which records the sparsity...

Evaluation criteria on the design for assimilating remote sensing data using variational approaches

Remote sensing, as a powerful tool for monitoring atmospheric phenomena, has been playing an increasingly important role in inverse modeling. Remote sensing instruments measure quantities that often combine several state variables as one. This creates very strong correlations between the state variables that share the same observation variable....

Estimation of volcanic ash emissions through assimilating satellite data and ground-based observations

In this paper, we reconstruct the vertical profile of volcanic ash emissions by assimilating satellite data and ground-based observations using a modified trajectory-based 4D-Var (Trj4DVar) approach. In our previous work, we found that the lack of vertical resolution in satellite ash column data can result in a poor estimation of the injection...