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Homborg, A.M. (author), Mol, J.M.C. (author), Tinga, Tiedo (author)This paper for the first time treats the interpretation of electrochemical noise time-frequency spectra as an image classification problem. It investigates the application of a convolutional neural network (CNN) for deep learning image classification of electrochemical noise time-frequency transient information. Representative slices of these...journal article 2024
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Imani, Amin (author), Rahimi, E. (author), Lekka, Maria (author), Andreatta, Francesco (author), Magnan, Michele (author), Gonzalez Garcia, Y. (author), Mol, J.M.C. (author), Raman, R. K. Singh (author), Fedrizzi, Lorenzo (author), Asselin, Edouard (author)Mg and its alloys are promising biodegradable materials for orthopedic implants and cardiovascular stents. The first interactions of protein molecules with Mg alloy surfaces have a substantial impact on their biocompatibility and biodegradation. We investigate the early-stage electrochemical, chemical, morphological, and electrical surface...journal article 2024
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Li, Z. (author), Visser, Peter (author), Hughes, Anthony E. (author), Homborg, A.M. (author), Gonzalez Garcia, Y. (author), Mol, J.M.C. (author)The quest for novel alternatives to hexavalent-chromium-based corrosion inhibitors is of utmost significance and urgency. Strict international health and safety regulations, due to growing concerns regarding the impact of hexavalent chromium on human health and the environment, have pushed the commercial introduction of many alternative...journal article 2024
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Cornet, A.J. (author), Homborg, A.M. (author), Ravi Anusuyadevi, P. (author), 't Hoen-Velterop, L. (author), Mol, J.M.C. (author)Despite extensive research, eliminating hexavalent chromium-based inhibitors from aerospace coatings remains challenging due to a lack of understanding of coating degradation during aircraft service. This study addresses the issue by investigating the protective mechanisms and aging processes of chromate-containing coatings on aircraft...journal article 2024
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Mopon, M. (author), Mol, J.M.C. (author), Garcia, Santiago J. (author)Understanding how late an inhibitor can be released once corrosion initiated without compromising corrosion protection may help in developing more efficient anticorrosion coatings. We explored this idea through time-controlled Ce(NO<sub>3</sub>)<sub>3</sub> availability to AA2024-T3 immersed in 0.05 M NaCl. Ce(NO<sub>3</sub>)<sub>3</sub> was...journal article 2024
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Gao, Yu (author), Zhang, Jingru (author), Wang, Donglei (author), Fan, Jiaxin (author), Mol, J.M.C. (author), Wang, Fuhui (author), Zhang, Danni (author), Xu, Dake (author)Microbially influenced corrosion (MIC) of metals exerts a negative effect on the marine environment and causes a great loss of marine facilities. Corrosion prevention in an eco-friendly and sustainable way is a difficult problem to address, especially in the marine environment. In this work, Nocardiopsis dassonville, a corrosive bacteria...journal article 2024
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Liu, M. (author), Zhu, Jia-Ning (author), Popovich, V. (author), Borisov, E. (author), Mol, J.M.C. (author), Gonzalez Garcia, Y. (author)Electrochemical tests and surface analysis measurements were performed to study the corrosion behavior in a 0.9 wt.% NaCl solution at 37 °C of three NiTi shape memory alloys fabricated by laser-powder bed fusion (L-PBF). The passive film characteristics and corrosion resistance of L-PBF NiTi showed different features as a function of their...journal article 2023
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Li, Z. (author), Homborg, A.M. (author), Gonzalez Garcia, Y. (author), Visser, Peter (author), Soleimani, M. (author), Mol, J.M.C. (author)The influence of ageing under ambient conditions on the corrosion protective behaviour of a lithium-based conversion layer on AA2024-T3 is studied in this work. Conversion layers aged at ambient conditions for relatively short times (0 h and 4 h), show an initial high degree of corrosion inhibition but a much lower protectiveness after the...journal article 2023
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Rahimi, E. (author), Sanchis-Gual, Roger (author), Chen, Xiangzhong (author), Imani, Amin (author), Gonzalez Garcia, Y. (author), Asselin, Edouard (author), Mol, J.M.C. (author), Fedrizzi, Lorenzo (author), Pané, Salvador (author), Lekka, Maria (author)The last two decades have witnessed the emergence of micro- and nanoswimmers (MNSs). Researchers have invested significant efforts in engineering motile micro- and nanodevices to address current limitations in minimally invasive medicine. MNSs can move through complex fluid media by using chemical fuels or external energy sources such as...review 2023
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Liu, M. (author), Zhu, Jia-Ning (author), Popovich, V. (author), Borisov, E. (author), Mol, J.M.C. (author), Gonzalez Garcia, Y. (author)Electrochemical tests and surface analysis were applied to study the corrosion behavior and passive film characteristics of three-dimensional-printed NiTi shape memory alloys fabricated by laser-powder bed fusion (L-PBF) in artificial saliva at 37 °C. The passivity of L-PBF NiTi shows to be influenced by the process parameters and resulting...journal article 2023
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Aghaeian, S. (author), Norouzi, F. (author), Sloof, W.G. (author), Mol, J.M.C. (author), Bottger, A.J. (author)The parabolic growth rate constant (k<sub>p</sub>) of high-temperature oxidation of steels is predicted via a data analytics approach. Four machine learning models including Artificial Neural Networks, Random Forest, k-Nearest Neighbors, and Support Vector Regression are trained to establish the relations between the input features ...journal article 2023
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Ma, Jinbo (author), Dai, Jiaxin (author), Guo, Xin (author), Fu, Dongmei (author), Ma, Lingwei (author), Keil, Patrick (author), Mol, J.M.C. (author), Zhang, Dawei (author)Following the construction of a dataset of cross-category corrosion inhibitors at different concentrations based on 1241 data from 184 research papers, a performance prediction model incorporating 2D–3D molecular graph representation and corrosion inhibitor concentration information was established. This model was shown to effectively predict...journal article 2023
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Liu, Tong (author), Zhang, Dawei (author), Zhang, Rongjun (author), Wang, Jinke (author), Ma, Lingwei (author), Keil, Patrick (author), Mol, J.M.C. (author), Li, Xiaogang (author)Organic coatings are one of the most used and versatile technologies to mitigate corrosion of metals. However, organic coatings are susceptible to defects and damages that may not be easily detected. If not repaired timely, these defects may develop into major coating failures due to corrosion occurring in the damaged region, thereby limiting...journal article 2023
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del Olmo, R. (author), López, E. (author), Matykina, E. (author), Tiringer, U. (author), Mol, J.M.C. (author), Mohedano, M. (author), Arrabal, R. (author)Plasma electrolytic oxidation (PEO) has been targeted as an eco-friendly alternative technology to conventional chromic acid anodizing (CAA) for corrosion protection of aluminium alloys in the aircraft industry. However, conventional PEO technology implies high energy consumption. Flash-PEO coatings (≤10 μm) produced in short treatment times ...journal article 2023
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Mousavi, M. (author), Kosari, A. (author), Mol, J.M.C. (author), Gonzalez Garcia, Y. (author)Electroless nickel (Ni) immersion gold (Au), commonly referred to by the acronym ENIG, is the most common protective coating applied on the exposed copper (Cu) traces of printed circuit boards (PCBs). In this work, we elucidate the local corrosion mechanism of the ENIG-Cu system by applying microscopic, surface analysis and electrochemical...journal article 2022
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Huang, Luyao (author), Chang, Weiwei (author), Zhang, Dawei (author), Huang, Ye (author), Li, Z. (author), Lou, Yuntian (author), Qian, Hongchang (author), Jiang, Chengying (author), Li, Xiaogang (author), Mol, J.M.C. (author)The influence of outward extracellular electron transfer (EET) of Pseudomonas aeruginosa in accelerating corrosion of 304 stainless steel was investigated. With less NO<sub>3</sub><sup>−</sup> available as electron acceptor, P. aeruginosa biofilm accelerated the pitting corrosion. The ICP-MS and XPS results indicated that P. aeruginosa...journal article 2022
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Zhou, Enze (author), Li, Feng (author), Zhang, Dawei (author), Xu, Dake (author), Li, Zhong (author), Jia, Ru (author), Song, Hao (author), Gu, Tingyue (author), Homborg, A.M. (author), Mol, J.M.C. (author)Shewanella oneidensis MR-1 is an attractive model microbe for elucidating the biofilm-metal interactions that contribute to the billions of dollars in corrosion damage to industrial applications each year. Multiple mechanisms for S. oneidensis-enhanced corrosion have been proposed, but none of these mechanisms have previously been rigorously...journal article 2022
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Li, Z. (author), Homborg, A.M. (author), Gonzalez Garcia, Y. (author), Kosari, A. (author), Visser, Peter (author), Mol, J.M.C. (author)The formation process of a lithium-based conversion layer on AA2024-T3 and its corrosion protective behavior are studied using electrochemical noise (EN). Wavelet transform, as well as noise resistance analysis, have been employed to interpret the EN data. The EN data confirmed five different stages during the conversion layer growth,...journal article 2022
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Chang, Weiwei (author), Li, Yangyang (author), Li, Z. (author), Lou, Yuntian (author), Cui, Tianyu (author), Qian, Hongchang (author), Mol, J.M.C. (author), Zhang, Dawei (author)The microbiologically influenced corrosion of pure iron was investigated in the presence of Shewanella oneidensis MR-1 with various levels of exogenous riboflavin (RF) serving as electron shuttles for extracellular electron transfer (EET). With more RF available, a larger and denser phosphate layer was formed on the surface of pure iron by...journal article 2022
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Dai, Jiaxin (author), Fu, Dongmei (author), Song, Guangxuan (author), Ma, Lingwei (author), Guo, Xin (author), Mol, J.M.C. (author), Cole, Ivan (author), Zhang, Dawei (author)Current experimental verification, computational modeling, and machine learning methods for predicting corrosion inhibition efficiency (IE) are limited to specific inhibitor categories with high cost and poor generalization. In this study, a cross-category corrosion inhibitor dataset is constructed and a three-level direct message passing...journal article 2022