Dynamic Growth of Macroscopically Structured Supramolecular Hydrogels through Orchestrated Reaction-Diffusion

Living organisms are capable of dynamically changing their structures for adaptive functions through sophisticated reaction-diffusion processes. Here we show how active supramolecular hydrogels with programmable lifetimes and macroscopic structures can be created by relying on a simple reaction-diffusion strategy. Two hydrogel precursors ...

Effects of microporous layer on electrolyte flooding in gas diffusion electrodes and selectivity of CO₂ electrolysis to CO

Understanding the relationship between gas diffusion electrode (GDE) structures and the performance of electrochemical CO₂ reduction reaction (CO₂RR) is crucial to developing industrial-scale technologies to convert CO₂ to valuable products. We studied how the microporous layer (MPL) on GDE's coated with...

Electrochemical CO₂ reduction in membrane-electrode assemblies

Electrochemical conversion of gaseous CO₂ to value-added products and fuels is a promising approach to achieve net-zero CO₂ emission energy systems. Significant efforts have been achieved in the design and synthesis of highly active and selective electrocatalysts for this reaction and their reaction mechanism. To perform...

Regulating the reaction zone of electrochemical CO₂ reduction on gas-diffusion electrodes by distinctive hydrophilic-hydrophobic catalyst layers

Regulating the rational wettability on gas-diffusion electrodes (GDEs) plays a pivotal role to improve the efficiency of CO₂RR via fine-tuning the reaction zone and boosting the formation of triple-phase interfaces. Herein, we present a wettability regulation strategy that modulates the triple-phase reaction zone in the catalyst...

Interactions between Diffuse Light and Cucumber (Cucumis sativus L.) Canopy Structure, Simulations of Light Interception in Virtual Canopies

Plant photosynthesis and biomass production are associated with the amount of intercepted light, especially the light distribution inside the canopy. Three virtual canopies (n = 80, 3.25 plants/m2) were constructed based on average leaf size of the digitized plant structures: ‘small leaf’ (98.1 cm2), ‘medium leaf’ (163.0 cm2) and ‘big leaf’ (241...

Continuum percolation threshold and ionic diffusivity of porous media consisting of asymmetrical ovoidal pores

Porous networks provide the main transport channels to the active media, which will damage the microstructure and then lead to a subsequent reduction in the strength, serviceability and aesthetic of porous materials. The connectivity of the porous network plays an essential role in the transport properties of these active media. In statistic...

Longitudinal diffusion MRI analysis using Segis-Net: A single-step deep-learning framework for simultaneous segmentation and registration

This work presents a single-step deep-learning framework for longitudinal image analysis, coined Segis-Net. To optimally exploit information available in longitudinal data, this method concurrently learns a multi-class segmentation and nonlinear registration. Segmentation and registration are modeled using a convolutional neural network and...

Neuro4Neuro: A neural network approach for neural tract segmentation using large-scale population-based diffusion imaging

Subtle changes in white matter (WM) microstructure have been associated with normal aging and neurodegeneration. To study these associations in more detail, it is highly important that the WM tracts can be accurately and reproducibly characterized from brain diffusion MRI. In addition, to enable analysis of WM tracts in large datasets and in...

Revealing the Impact of Space-Charge Layers on the Li-Ion Transport in All-Solid-State Batteries

The influence of space-charge layers on the ionic charge transport over cathode-solid electrolyte interfaces in all-solid-state batteries remains unclear because of the difficulty to unravel it from other contributions to the ion transport over the interfaces. Here, we reveal the effect of the space-charge layers by systematically tuning the...

The Improvement of Oxidation Resistance of a Re-Based Diffusion Barrier/Ni–Al Coating on the Single-Crystal Ni-Based TMS-82+ Superalloy

Oxidation behavior of a Re-based diffusion barrier/Ni–Al coated single-crystal (SC) Ni-based TMS-82+ superalloy was studied to compare with those of the base and Ni–Al coated superalloys under cyclic air at 1150 °C for 200 h. The base superalloy showed a negative mass gain due to extensive oxide spallation, and the Ni–Al coated superalloy...

Improvement of the Oxidation Resistance of the Single-Crystal Ni-Based TMS-82+ Superalloy by Ni–Al Coatings with/without the Diffusion Barrier

Oxidation behavior of the uncoated base, Ni–Al coated and Re–Cr-Ni plus Ni–Al coated single-crystal (SC) Ni-based TMS-82+ superalloy is studied under cyclic air at 900ºC for 200 h to assess the oxidation resistance. Regardless of the coating processing, Ni–Al coating is effective in improving the oxidation resistance due to the formation of a...

A Hybrid Five-Point Finite Difference Scheme for Convection-Diffusion Equations

In this paper, some five-point finite difference schemes for steady convection-diffusion problems are presented. To begin with, we use the finite volume method (FVM) to discretize the convection-diffusion equation. After that, we present two five-point difference schemes for the approximation of the first order derivatives on faces, one of which...