The main bottleneck during the manufacture of complex geometry thin-walled GFRC structures is the time taken to make the timber or CNC machined moulds for each panel. Complex geometries are comprised of many unique panel forms and the extensive time and high costs of their manufacture often prevents their architectural intent from being fully realised. A novel mould-making process is proposed that uses a state-of-the-art flexible table with computer-controlled actuators to create free-formed geometry, fast-curing, dual-density, polyurethane moulds. This mould-making process was successfully tested by using sprayed GFRC to manufacture 9 different double curved intermediate moulds for a 10 m high GFRC self-supporting, thin-walled hyperbolic shell, with 12 mm thick panels at the base of the structure. The completed structure showcased the effectiveness of the novel mould-making process by reducing the production time from an estimated 100 days to 10 days. The primary outcome was the development and application of a new manufacturing method capable of casting complex geometry thin-walled GFRC panels with good surface quality that was suited to more rapid, cost-effective and automated large-scale production.@en