Nonlinear responses of nanoparticles induce enlightening phenomena in optical tweezers. With the gradual increase in optical intensity, effects from saturable absorption (SA) and reverse SA (RSA) arise in sequence and thereby modulate the nonlinear properties of materials. In current nonlinear optical traps, however, the underlying physical mechanism is mainly confined within the SA regime because threshold values required to excite the RSA regime are extremely high. Herein, we demonstrate, both in theory and experiment, nonlinear optical tweezing within the RSA regime, proving that a fascinating composite trapping state is achievable at ultrahigh intensities through an optical force reversal induced through nonlinear absorption. Integrated results help in perfecting the nonlinear optical trapping system, thereby providing beneficial guidance for wider applications of nonlinear optics.

A new type of radially polarized (RP) cosine-Gaussian (CG) field is proposed. Through the analytical model, it is found that such RP CG beam exhibits completely different focusing properties from the reported RP plane waves. More importantly, a stable three-dimensional trap of Rayleigh particle accompanied by a subwavelength spin motion can be easily achieved using this RP CG beam.

Single molecule detection and analysis play important roles in many current biomedical researches. The deep-nanoscale hotspots, being excited and confined in a plasmonic nanocavity, make it possible to simultaneously enhance the nonlinear light-matter interactions and molecular Raman scattering for label-free detections. Here, we theoretically show that a nanocavity formed in a tip-enhanced Raman scattering (TERS) system can also achieve valid optical trapping as well as TERS signal detection for a single molecule. In addition, the nonlinear responses of metallic tip and substrate film can change their intrinsic physical properties, leading to the modulation of the optical trapping force and the TERS signal. The results demonstrate a new degree of freedom brought by the nonlinearity for effectively modulating the optical trapping and Raman detection in single molecule level. This proposed platform also shows a great potential in various fields of research that need high-precision surface imaging.

Since the invention of optical tweezers, optical manipulation has advanced significantly in many applications, including atomic physics, biochemistry and soft matter physics. Here, we propose a method to trap metallic particles with adjustable trapping range in the transverse plane with the help of customized field. By tailoring the polarization state of the incident field, the focal field with elongation in the direction perpendicular to optical axis can be turned in the 4π focusing system. As a result, optical trapping with tunable trapping range is possible when the metallic particle is interacted with such customized field.

We propose a simple method to control the move and elongation of focus along the optical axis in a high-numerical aperture focusing system. By introducing the optical degree of freedom of polarization in the radial direction, a tunable focal shift and elongation of focus are achieved simply by tailoring the polarization index and the topological charge of vortex phase, without the need of additional modulations of amplitude or diffractive optical elements. These findings may be of help in the applications like optical micro-manipulation, laser processing, and imaging.

As an intrinsic attribute of light, the spin angular momentum (SAM) of photons has aroused considerable attention because of the fascinating properties emerging from light–matter interactions. We show that a diffraction-limited focal field with a steerable photonic spin structure in three dimensions can be produced under a 4π microscopic system. This is achieved by focusing two counter-propagating configurable vector beams produced in the coherent superposition of three different beams with x-polarization, y-polarization, and radial-polarization. By altering the amplitude factors of these resultant beams, the ratios between the three mutually orthogonal polarized components can be freely tuned within the focal plane, thereby allowing dynamic control over the spin orientation and ellipticity of the tightly focused optical field. The results demonstrated in this paper may find applications in spin-controlled nanophotonics.