In this work, shear-thickening-gel applied CFRP (SACFRP) composite laminates were developed to enhance the impact resistance of the composites under low-velocity impact (LVI) conditions, where the incorporated shear thickening gel (STG) worked as the interphase material between fibres and resin matrix. To analyse the effects of STG in its composites, static tensile and shear tests were first conducted on longitudinally and transversely positioned unidirectional (UD) SACFRP and its CFRP reference, respectively. Experimental results indicated that the corresponding reduction of the resin matrix due to the incorporation of the relatively soft STG weakened the interlaminar behaviour of the SACFRP laminates during static mechanical tests. However, the transverse tensile toughness of the SACFRP exhibited a remarkable 139 % improvement compared to the CFRP reference, demonstrating significant interfacial toughening of the developed composites, as verified through SEM analysis. To leverage the effects of the STG on the composites, this work modified the stacking sequences of SACFRP laminates. LVI tests and recurring LVI tests demonstrated the substantial improvement of impact performance for layup-designed SACFRP laminates since the impact-resistant mechanism transitioned from the local damage of CFRPs to the global flexural behaviour of SACFRPs. Timoshenko's analytical model validated the resistant mechanism transition of layup-designed SACFRP during LVI tests. Therefore, the SACFRP laminates with modified stacking sequences demonstrate outstanding potential for use under extreme loading conditions involving complex and unavoidable impacts, highlighting their broad applicability across various industries.

Conventional carbon fiber-reinforced polymers (CFRPs) are highly susceptible to low-velocity impact (LVI) from sharp objects due to their inherent brittleness. To address this critical limitation, an innovative shear thickening gel (STG) was incorporated into CFRP through a bespoke fabrication process, resulting in the STG-applied CFRP (SACFRP). LVI tests revealed that specific impact strength of the SACFRP increased significantly by 267 % compared to the reference CFRP fabricated with the same carbon fibers and epoxy resin but without STG. Moreover, the SACFRP achieved the specific impact strength of 202 J m/kg, substantially exceeding that of other representative carbon or glass fiber-reinforced polymers. Damage analysis and Timoshenko's theoretical study highlighted distinct failure mechanisms between the SACFRP that exhibited thin-plate elastic flexure and the CFRP that experienced brittle impact failure under LVI. Additionally, ultrasonic C-scan results demonstrated enlarged effective impact-resistant area in the SACFRP due to the viscoelasticity and shear-thickening behavior of the integrated STG, facilitating energy dissipation and reducing brittleness of the composite. In summary, this work presents the manufacturing method of an innovative SACFRP composite and demonstrates its outstanding impact resistance, marking the significant advancement in development of high-performance composites.