This paper presents a method to control chaotic behavior of a typical Smart Grid based on generalized fuzzy hyperbolic model (GFHM). As more and more distributed generations (DG) are incorporated into the Smart Grid, the chaotic behavior occurs increasingly. To verify the behavior, a dynamic model which describes a power system with DG is presented firstly. Then, the simulation result shows that the power system can lead to chaos under certain initial conditions. Based on the universal approximation of GFHM, we confirm that the chaotic behavior could be suppressed by a new controller, which is designed by means of solving a linear matrix inequality (LMI). This approach could make a good application to suppress the chaos in Smart Grid. Finally, a numerical example is given to demonstrate the effectiveness of the proposed chaotic suppression strategy.