LH

Lingtjien Hong

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Journal article (2020) - Dion J. Koeze, Lingtjien Hong, Abhishek Kumar, Brian P. Tighe
Numerous soft materials jam into an amorphous solid at a high packing fraction. This nonequilibrium phase transition is best understood in a model system where particles repel when they overlap. Recently, however, it was shown that introducing any finite amount of attraction between particles changes the universality class of the transition. The properties of this "sticky jamming"class remain almost entirely unexplored. We use molecular dynamics simulations and scaling analysis to determine the shear modulus, bulk modulus, and coordination of marginal solids close to the sticky jamming point. Each observable differs not just quantitatively but also qualitatively from the purely repulsive case. ...
While jamming is best understood in the context of purely repulsive soft spheres, emulsions and other experimental realizations of the soft sphere model commonly display weakly cohesive forces. We perform simulations of soft spheres with a finite-ranged attractive tail in the pair potential. The resulting attractive soft sphere packings can be stable at volume fractions below the purely repulsive jamming point. These new jammed states have counter-intuitive properties -- for example, while attraction introduces tensile forces, their presence leads to an increase in the compressive stress. We use critical scaling analysis to characterize the geometry and mechanics of attractive soft sphere packings as a function of both the volume fraction and the range of the attractive interaction. ...