Molecular tagging is used to study the dispersion and deformation of patterns written in turbulent air. The writing is done by fusing O2 and N2 molecules into NO in the focus of a strong ultraviolet laser beam. By crossing several of these laser beams, patterns that have both small and large scales can be painted. The patterns are visualized a while later by inducing fluorescence of the NO molecules with a second UV laser and registering the image. The width of the lines that make the pattern is approximately 50μm, a few times the Kolmogorov length η, the smallest length scale in turbulence, while the largest size of the patterns (≈4mm) is inside the inertial range of the used turbulent jet flow. At small scales molecular clouds disperse under the joint action of molecular diffusion and turbulence. The experiments reveal this highly nontrivial interaction. At inertial-range scales (≈200η) we verify the Batchelor dispersion of objects whose size is inside the inertial range. Patterns are compressible objects and spontaneously develop concentration fluctuations. We show for the first time the nontrivial statistical properties of these fluctuations. Finally, we use the information in written and deformed lines to quantify turbulent intermittency, obtaining results that agree with the established scaling anomaly of velocity structure functions.

We study the dispersion of tiny molecular clouds in turbulence by writing patterns in turbulent air and following their deformation in time. The writing is done by fusing O2 and N2 molecules into NO in the focus of a strong ultraviolet laser beam. By crossing several of these laser beams, patterns that have both small and large scales can be painted. The patterns are visualized a while later by inducing fluorescence of the NO molecules with a second UV laser and registering the image. The width of the lines that make the pattern is approximately 50 μm, a few times the Kolmogorov length η, the smallest length scale in turbulence, while the overall size of the patterns (≈4 mm) is inside the inertial range of the used turbulent jet flow. At small scales molecular clouds disperse under the joint action of molecular diffusion and turbulence. The experiments reveal for the first time this subtle, yet very important interaction. At macroscales (≈200 η) we verify the Batchelor dispersion of objects whose size is inside the inertial range; however, the expected influence of molecular diffusion is smaller than the accuracy of the experiments.

We present a new technique to study preferential concentration of droplets in a turbulent air flow. Preferential concentration is the tendency of droplets to cluster in regions of strain, while avoiding regions of rotation. We study the properties of the droplet concentration field in zero mean flow turbulence that was created using an array of synthetic jets. The droplets are made of a phosphorescent solution of Europium chelate. They are excited by a laser sheet from a pulsed UV laser, after which the glowing droplets are followed using a high-speed intensified camera. We quantify preferential concentration through measurement of moments of the coarse-grained local droplet density. At the Stokes numbers studied (St≈2) the fractal dimension, a scaling property of this coarse-grained density field, points to clustering. Clustering is a consequence of the compressibility of the droplet velocity field. We also quantify the dynamical behavior of clustering by moving with this velocity field. We find a preference for clustering in the Lagrangian frame during the time interval set by the decay of the phosphorescence.