Recovery of rare earths from glass polishing waste for the production of aluminium-rare earth alloys

Journal Article (2021)
Authors

Chenna Borra ((OLD) MSE-1, Indian Institute of Technology Madras)

Thijs J. H. Vlugt (TU Delft - Engineering Thermodynamics)

Yong xiang Yang (TU Delft - Team Yongxiang Yang)

Jeroen Spooren (Vlaamse Instelling voor Technologisch Onderzoek)

Peter Nielsen (Vlaamse Instelling voor Technologisch Onderzoek)

Murugaiyan Amirthalingam (Indian Institute of Technology Madras)

Sven Erik Offerman (TU Delft - Team Erik Offerman)

Research Group
Engineering Thermodynamics
Copyright
© 2021 C.R. Borra, T.J.H. Vlugt, Y. Yang, Jeroen Spooren, Peter Nielsen, Murugaiyan Amirthalingam, S.E. Offerman
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Publication Year
2021
Language
English
Copyright
© 2021 C.R. Borra, T.J.H. Vlugt, Y. Yang, Jeroen Spooren, Peter Nielsen, Murugaiyan Amirthalingam, S.E. Offerman
Research Group
Engineering Thermodynamics
Bibliographical Note
Green Open Access added to TU Delft Institutional Repository 'You share, we take care!' - Taverne project https://www.openaccess.nl/en/you-share-we-take-care Otherwise as indicated in the copyright section: the publisher is the copyright holder of this work and the author uses the Dutch legislation to make this work public.@en
Volume number
174
DOI:
https://doi.org/10.1016/j.resconrec.2021.105766
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Abstract

The circular economy demands waste utilization for the production of high-value products, and this requires the development of novel processing routes. In this study, rare earth (La and Ce) oxides were completely (>99%) recovered from polishing waste by a combined novel reductive acid leaching and alkali treatment process. About 70% of rare earths were dissolved during the first leaching step. The undissolved rare earth compounds are converted to oxides/hydroxides by alkali treatment and dissolved in the acid solution – the 2nd leaching step – for the complete recovery of rare earths. The recovered rare earth oxides were used for producing in-situ high-value Al-La-Ce alloys with fused salt electrolysis. Mechanical properties of our Al-La-Ce alloys are similar to the known high temperature Al-Ce alloys. This development of new alloys by our novel process helps in utilization of both overproduced primary La and Ce oxides as well as La and Ce recovered from polishing waste.

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