Spin excitations in an all-organic double quantum dot molecule

Journal Article (2016)
Author(s)

M. Koole (TU Delft - QN/van der Zant Lab)

Jan C. Hummelen (Rijksuniversiteit Groningen)

H.S.J. van der Zant (TU Delft - QN/van der Zant Lab)

Research Group
QN/van der Zant Lab
Copyright
© 2016 M. Koole, Jan C. Hummelen, H.S.J. van der Zant
DOI related publication
https://doi.org/10.1103/PhysRevB.94.165414
More Info
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Publication Year
2016
Language
English
Copyright
© 2016 M. Koole, Jan C. Hummelen, H.S.J. van der Zant
Research Group
QN/van der Zant Lab
Issue number
16
Volume number
94
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Abstract

We realize a strongly coupled double quantum dot in a single all-organic molecule by introducing a nonconjugated bridge in between two identical conjugated moieties. Spin-1/2 Kondo and Kondo enhanced low-energy excitations for, respectively, the odd and even electron occupation are observed in off-resonant transport. The ground state in the even occupation can be the singlet or the triplet state varying between samples. This observation suggests that both antiferromagnetic and ferromagnetic interactions between spins are of the same order of magnitude.