Single-Crystal Rutile TiO 2 Nanocylinders are Highly Effective Transducers of Optical Force and Torque

Journal Article (2019)
Author(s)

S. Ha (TU Delft - BN/Nynke Dekker Lab, Kavli institute of nanoscience Delft)

Y. Tang (TU Delft - ImPhys/Optics)

Maarten M. van Oene (Kavli institute of nanoscience Delft, Student TU Delft)

R. Janissen (Kavli institute of nanoscience Delft, TU Delft - BN/Nynke Dekker Lab)

R.M. Dries (Kavli institute of nanoscience Delft, TU Delft - BN/Marileen Dogterom Lab)

Belén Solano Hermosilla (TU Delft - BN/Nynke Dekker Lab)

AJL Adam (TU Delft - ImPhys/Optics)

N.H. Dekker (TU Delft - BN/Nynke Dekker Lab, Kavli institute of nanoscience Delft)

Research Group
ImPhys/Optics
Copyright
© 2019 S. Ha, Y. Tang, M.M. van Oene, R. Janissen, R.M. Dries, B.P. Solano Hermosilla, A.J.L. Adam, N.H. Dekker
DOI related publication
https://doi.org/10.1021/acsphotonics.9b00220
More Info
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Publication Year
2019
Language
English
Copyright
© 2019 S. Ha, Y. Tang, M.M. van Oene, R. Janissen, R.M. Dries, B.P. Solano Hermosilla, A.J.L. Adam, N.H. Dekker
Research Group
ImPhys/Optics
Issue number
5
Volume number
6
Pages (from-to)
1255-1265
Reuse Rights

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Abstract


Optical trapping of (sub)micron-sized particles is broadly employed in nanoscience and engineering. The materials commonly employed for these particles, however, have physical properties that limit the transfer of linear or angular momentum (or both). This reduces the magnitude of forces and torques, and the spatiotemporal resolution, achievable in linear and angular traps. Here, we overcome these limitations through the use of single-crystal rutile TiO
2
, which has an exceptionally large optical birefringence, a high index of refraction, good chemical stability, and is amenable to geometric control at the nanoscale. We show that rutile TiO
2
nanocylinders form powerful joint force and torque transducers in aqueous environments by using only moderate laser powers to apply nN·nm torques at kHz rotational frequencies to tightly trapped particles. In doing so, we demonstrate how rutile TiO
2
nanocylinders outperform other materials and offer unprecedented opportunities to expand the control of optical force and torque at the nanoscale.