Sustainable advanced wastewater treatment via photoelectrocatalytic oxidation

insights from life cycle assessment

Journal Article (2025)
Author(s)

Gema Amaya Santos (University College London)

Agha Zeeshan Ali (Avans Hogeschool Breda, TU Delft - Civil Engineering & Geosciences)

Paola Lettieri (University College London)

Research Group
Sanitary Engineering
DOI related publication
https://doi.org/10.1038/s41545-025-00522-x Final published version
More Info
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Publication Year
2025
Language
English
Research Group
Sanitary Engineering
Journal title
npj Clean Water
Issue number
1
Volume number
8
Article number
94
Downloads counter
39
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Abstract

This study presents a life cycle assessment (LCA) of a scaled-up photoelectrocatalytic (PEC) oxidation system for wastewater treatment, modelled using computational fluid dynamics (CFD). The system used a BiVO4/TiO2-GO photoanode for solar-driven degradation of micropollutants. The LCA assesses energy use, resource demand, and emissions to evaluate the system’s sustainability in line with EU wastewater regulations. Compared to a full-scale ozonation plant in the Netherlands, the PEC system shows superior environmental performance during operation and end-of-life phases, despite higher construction impacts. Solar energy use and potential material reuse drive these advantages. A comparison with theoretical pilot-scale oxidation technologies from literature adds depth, though the study acknowledges limitations such as micropollutant variability and wastewater complexity. Overall, the findings highlight PEC oxidation’s promise as a sustainable and effective approach for micropollutant removal in water treatment.