Print Email Facebook Twitter Rayleigh-Brillouin light scattering spectra of CO2 from molecular dynamics Title Rayleigh-Brillouin light scattering spectra of CO2 from molecular dynamics Author Jamali, S.H. (TU Delft Engineering Thermodynamics) de Groen, M. (TU Delft Engineering Thermodynamics) Moultos, O. (TU Delft Engineering Thermodynamics) Hartkamp, Remco (TU Delft Complex Fluid Processing) Vlugt, T.J.H. (TU Delft Engineering Thermodynamics) Ubachs, Wim (Vrije Universiteit Amsterdam) van de Water, W. (TU Delft Fluid Mechanics) Date 2019 Abstract Rayleigh-Brillouin light scattering spectra of CO2 at ultraviolet wavelengths are computed from molecular dynamics which depends on intermolecular potentials only. We find excellent agreement with state of the art experimental data. This agreement was reached in a minimal computational box with sides one scattering wavelength long and integrating the classical trajectories over 20 ns. We also find complete consistency with models based on kinetic theory, which take known values of the transport coefficients as input. To reference this document use: http://resolver.tudelft.nl/uuid:682b610b-bcef-4a2a-9b1c-7a2ce10af3ae DOI https://doi.org/10.1063/1.5110676 Embargo date 2020-02-14 ISSN 0021-9606 Source Journal of Chemical Physics, 151 (6) Bibliographical note Green Open Access added to TU Delft Institutional Repository ‘You share, we take care!’ – Taverne project https://www.openaccess.nl/en/you-share-we-take-care Otherwise as indicated in the copyright section: the publisher is the copyright holder of this work and the author uses the Dutch legislation to make this work public. Part of collection Institutional Repository Document type journal article Rights © 2019 S.H. Jamali, M. de Groen, O. Moultos, Remco Hartkamp, T.J.H. Vlugt, Wim Ubachs, W. van de Water Files PDF 1.5110676_1.pdf 1.77 MB Close viewer /islandora/object/uuid:682b610b-bcef-4a2a-9b1c-7a2ce10af3ae/datastream/OBJ/view