Enhancing the durability of Pt nanoparticles for water electrolysis using ultrathin SiO2 layers

Extending the lifetime of electrocatalytic materials is a major challenge in electrocatalysis. Here, we employ atomic layer deposition (ALD) to coat the surface of carbon black supported platinum nanoparticles (Pt/CB) with an ultra-thin layer of silicon dioxide (SiO2) to prevent deactivation of the catalyst during H2 evolution. Our results show...

Tuning the Properties of N-Doped Biochar for Selective CO₂ Electroreduction to CO

Nitrogen-doped (N-doped) carbon catalysts have been widely studied for electrochemical CO₂ reduction to CO. However, the correlation between the physicochemical properties of N-doped carbon catalysts and their electrocatalytic performance for the CO₂RR is still unclear. Herein, a series of N-doped biochar catalysts with...

Unravelling the Effect of Activators used in The Synthesis of Biomass-Derived Carbon Electrocatalysts on the Electrocatalytic Performance for CO₂ Reduction

N-doped carbon materials can be efficient and cost-effective catalysts for the electrochemical CO₂ reduction reaction (CO₂RR). Activators are often used in the synthesis process to increase the specific surface area and porosity of these carbon materials. However, owing to the diversity of activators and the differences...

Nanostructuring Pt-Pd Bimetallic Electrocatalysts for CO₂ Reduction Using Atmospheric Pressure Atomic Layer Deposition

Preparing supported nanoparticles with a well-defined structure, uniform particle size, and composition using conventional catalyst synthesis methods, such as impregnation, precipitation, and deposition-precipitation is challenging. Furthermore, these liquid phase methods require significant solvent consumption, which has sustainable issues...