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Lei, Yutian (author), Li, Zhen-Hua (author), Wang, H. (author), Wang, Qian (author), Peng, Guoqiang (author), Xu, Youkui (author), Zhang, Haihua (author), Wang, Gang (author), Ding, Liming (author), Jin, Zhiwen (author)Two-dimensional (2D) Dion-Jacobson (D-J)-type cesium lead iodide CsPbI <sub>3</sub> perform remarkably in terms of stability. However, the complex interactions between spacer and inorganic layers limit its excellent progress in perovskite solar cells (PSCs). Herein, starting from the considerable structural diversity of organic spacers, we...journal article 2022
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Wang, Shuo (author), Xu, Youkui (author), Wang, Qian (author), Zhou, Xufeng (author), Li, ZhenHua (author), Wang, Meng (author), Lei, Yutian (author), Zhang, Hong (author), Wang, H. (author), Jin, Zhiwen (author)Iodine vacancies and uncoordinated iodide ions of CsPbI<sub>3</sub> films are mainly responsible for nonradiative recombination. Here, we report a composition-engineering passivation method that through guanidium (GA<sup>+</sup>) and I<sup>−</sup> forms strong hydrogen bonds to passivate iodine vacancies and reduce defects. Both experimental...journal article 2022