Closing the Loop: Unexamined Performance Trade-Offs of Integrating Direct Air Capture with (Bi)carbonate Electrolysis

CO₂ from carbonate-based capture solutions requires a substantial energy input. Replacing this step with (bi)carbonate electrolysis has been commonly proposed as an efficient alternative that coproduces CO/syngas. Here, we assess the feasibility of directly integrating air contactors with (bi)carbonate electrolyzers by leveraging...

On the relation between antecedent basin conditions and runoff coefficient for European floods

The event runoff coefficient (i.e. the ratio between event runoff and precipitation that originated the runoff) is a key factor for understanding basin response to precipitation events. Runoff coefficient depends on precipitation intensity and duration but also on specific basin geohydrology attributes (including soil type, geology, land...

Perspective on satellite-based land data assimilation to estimate water cycle components in an era of advanced data availability and model sophistication

The beginning of the 21^st century is marked by a rapid growth of land surface satellite data and model sophistication. This offers new opportunities to estimate multiple components of the water cycle via satellite-based land data assimilation (DA) across multiple scales. By resolving more processes in land surface models and by...

An Agenda for Land Data Assimilation Priorities: Realizing the Promise of Terrestrial Water, Energy, and Vegetation Observations From Space

The task of quantifying spatial and temporal variations in terrestrial water, energy, and vegetation conditions is challenging due to the significant complexity and heterogeneity of these conditions, all of which are impacted by climate change and anthropogenic activities. To address this challenge, Earth Observations (EOs) of the land and...

Modeling the Local Environment within Porous Electrode during Electrochemical Reduction of Bicarbonate

The electrochemical reduction of bicarbonate to renewable chemicals without external gaseous CO2 supply has been motivated as a means of integrating conversion with upstream CO2 capture. The way that CO2 is formed and transported during CO2-mediated bicarbonate reduction in flow cells is profoundly different from conventional CO2 saturated...

Design and characterization of zero magnetic field chambers for high efficiency neutron polarization transport

Several methods of polarized neutron scattering call for a zero magnetic field (ZF) region to reduce magnetic field integral aberrations while preserving the neutron polarization. Though the design for large angle neutron scattering has been presented in various places, the design characterization and tuning has not been discussed before. In...

New capabilities in high-resolution neutron Larmor diffraction at ORNL

High resolution neutron Larmor diffraction using superconducting magnetic Wollaston prisms

The neutron Larmor diffraction technique has been implemented using superconducting magnetic Wollaston prisms in both single-arm and double-arm configurations. Successful measurements of the coefficient of thermal expansion of a single-crystal copper sample demonstrates that the method works as expected. The experiment involves a new method of...