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Wang, C. (author), Liu, M. (author), Bannenberg, L.J. (author), Zhao, C. (author), Thijs, M.A. (author), Boshuizen, B. (author), Ganapathy, S. (author), Wagemaker, M. (author)Lithium metal with its high theoretical capacity and low negative potential is considered one of the most important candidates to raise the energy density of all-solid-state batteries. However, lithium filament growth and its induced solid electrolyte decomposition pose severe challenges to realize a long cycle life. Here, dendrite growth in...journal article 2024
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Wang, Q. (author), Zhou, Dong (author), Zhao, C. (author), Wang, Jianlin (author), Guo, Hao (author), Wang, Liguang (author), Yao, Zhenpeng (author), Lu, Jun (author), Wagemaker, M. (author)Sodium-ion batteries have not only garnered substantial attention for grid-scale energy storage owing to the higher abundance of sodium compared with lithium, but also present the possibility of fast charging because of the inherently higher sodium-ion mobility. However, it remains a phenomenal challenge to achieve a combination of these...journal article 2024
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Wang, Q. (author), Zhou, Yunan (author), Wang, Xuelong (author), Guo, Hao (author), Gong, Shuiping (author), Yao, Zhenpeng (author), Ganapathy, S. (author), Zhao, C. (author), Wagemaker, M. (author)All-solid-state lithium batteries have attracted widespread attention for next-generation energy storage, potentially providing enhanced safety and cycling stability. The performance of such batteries relies on solid electrolyte materials; hence many structures/phases are being investigated with increasing compositional complexity. Among the...journal article 2024
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Wang, Q. (author), Zhao, C. (author), Yao, Zhenpeng (author), Wang, Jianlin (author), Wu, Fangting (author), Kumar, Sai Govind Hari (author), Ganapathy, S. (author), Eustace, S.J. (author), Wagemaker, M. (author)Developing liquid electrolytes with higher kinetics and enhanced interphase stability is one of the key challenges for lithium batteries. However, the poor solubility of lithium salts in solvents sets constraints that compromises the electrolyte properties. Here, it is shown that introducing multiple salts to form a high-entropy solution,...journal article 2023
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Liu, M. (author), Wang, C. (author), Zhao, C. (author), van der Maas, E.L. (author), Lin, Kui (author), Arszelewska, Violetta (author), Li, Baohua (author), Ganapathy, S. (author), Wagemaker, M. (author)The original version of this article contained errors in Figure 3a and Figure 3f. In Figure 3a, the activation energies (Ea) were calculated using a log scale instead of a logarithm ln scale. In Figure 3f, the y-axis interval was not properly selected. The correct y-axis interval in Figure 3f and the numerical values of the activation energy...journal article 2023
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Wang, Zaifa (author), Wang, Zhenyu (author), Xue, Dingchuan (author), Zhao, Jun (author), Zhang, Xuedong (author), Geng, Lin (author), Li, Yanshuai (author), Du, Congcong (author), Wagemaker, M. (author)The rock-salt phase (RSP) formed on the surface of Ni-rich layered cathodes in liquid-electrolyte lithium-ion batteries is conceived to be electrochemically "dead". Here we show massive RSP forms in the interior of LiNi<sub>x</sub>Mn<sub>y</sub>Co<sub>(1−x-y)</sub>O<sub>2</sub> (NMC) crystals in sulfide based all solid state batteries (ASSBs)...journal article 2023
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Wang, Q. (author), Zhao, C. (author), Wang, Jianlin (author), Yao, Zhenpeng (author), Wang, Shuwei (author), Kumar, Sai Govind Hari (author), Ganapathy, S. (author), Eustace, S.J. (author), Wagemaker, M. (author)High-entropy alloys/compounds have large configurational entropy by introducing multiple components, showing improved functional properties that exceed those of conventional materials. However, how increasing entropy impacts the thermodynamic/kinetic properties in liquids that are ambiguous. Here we show this strategy in liquid electrolytes...journal article 2023
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Liu, M. (author), Zhang, S. (author), van Eck, Ernst R.H. (author), Wang, C. (author), Ganapathy, S. (author), Wagemaker, M. (author)The development of commercial solid-state batteries has to date been hindered by the individual limitations of inorganic and organic solid electrolytes, motivating hybrid concepts. However, the room-temperature conductivity of hybrid solid electrolytes is still insufficient to support the required battery performance. A key challenge is to...journal article 2022
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Wang, Q. (author), Zhao, C. (author), Wang, Shuwei (author), Wang, Jianlin (author), Liu, M. (author), Ganapathy, S. (author), Bai, Xuedong (author), Li, Baohua (author), Wagemaker, M. (author)Improving the reversibility of lithium metal batteries is one of the challenges in current battery research. This requires better fundamental understanding of the evolution of the lithium deposition morphology, which is very complex due to the various parameters involved in different systems. Here, we clarify the fundamental origins of...journal article 2022
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Liu, M. (author), Wang, C. (author), Zhao, C. (author), van der Maas, E.L. (author), Lin, Kui (author), Arszelewska, Violetta (author), Li, Baohua (author), Ganapathy, S. (author), Wagemaker, M. (author)A key challenge for solid-state-batteries development is to design electrode-electrolyte interfaces that combine (electro)chemical and mechanical stability with facile Li-ion transport. However, while the solid-electrolyte/electrode interfacial area should be maximized to facilitate the transport of high electrical currents on the one hand,...journal article 2021
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Wang, C. (author), Liu, M. (author), Thijs, M.A. (author), Ooms, F.G.B. (author), Ganapathy, S. (author), Wagemaker, M. (author)Li metal batteries are being intensively investigated as a means to achieve higher energy density when compared with standard Li-ion batteries. However, the formation of dendritic and mossy Li metal microstructures at the negative electrode during stripping/plating cycles causes electrolyte decomposition and the formation of electronically...journal article 2021
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van der Jagt, R. (author), Vasileiadis, A. (author), Veldhuizen, H.V. (author), Ganapathy, S. (author), Habisreutinger, N.C.P. (author), van der Veen, M.A. (author), Wang, C. (author), Wagemaker, M. (author), van der Zwaag, S. (author), Nagai, A. (author)Covalent organic frameworks (COFs) are an emerging material family having several potential applications. Their porous framework and redox-active centers enable gas/ion adsorption, allowing them to function as safe, cheap, and tunable electrode materials in next-generation batteries, as well as CO2 adsorption materials for carbon-capture...journal article 2021
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Zhao, Chenglong (author), Yao, Zhenpeng (author), Wang, Qidi (author), Li, Haifeng (author), Wang, Jianlin (author), Liu, M. (author), Ganapathy, S. (author), Lu, Yaxiang (author), Wagemaker, M. (author)Layered Na-based oxides with the general composition of NaxTMO2 (TM: transition metal) have attracted significant attention for their high compositional diversity that provides tunable electrochemical performance for electrodes in sodium-ion batteries. The various compositions bring forward complex structural chemistry that is decisive for...journal article 2020
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Liu, M. (author), Wang, C. (author), Cheng, Z. (author), Ganapathy, S. (author), Haverkate, Lucas A. (author), Unnikrishnan, Sandeep (author), Wagemaker, M. (author)Solid-state lithium-metal batteries are considered to be promising candidates for next-generation high-energy density storage devices to power electrical vehicles. Critical challenges for solid-state lithium-metal batteries include the large morphological changes associated with the plating and stripping of lithium metal and decomposition of...journal article 2020
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Wang, Qidi (author), Yao, Zhenpeng (author), Zhao, Chenglong (author), Verhallen, T.W. (author), Tabor, Daniel P. (author), Liu, M. (author), Ooms, F.G.B. (author), Kang, Feiyu (author), Wagemaker, M. (author)Metallic lithium is a promising anode to increase the energy density of rechargeable lithium batteries. Despite extensive efforts, detrimental reactivity of lithium metal with electrolytes and uncontrolled dendrite growth remain challenging interconnected issues hindering highly reversible Li-metal batteries. Herein, we report a rationally...journal article 2020
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Zhao, Chenglong (author), Wang, Qidi (author), Yao, Zhenpeng (author), Wang, Jianlin (author), Sánchez-Lengeling, Benjamín (author), Ding, Feixiang (author), Qi, Xingguo (author), Lu, Yaxiang (author), Wagemaker, M. (author)Sodium-ion batteries have captured widespread attention for grid-scale energy storage owing to the natural abundance of sodium. The performance of such batteries is limited by available electrode materials, especially for sodium-ion layered oxides, motivating the exploration of high compositional diversity. How the composition determines the...journal article 2020
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Liu, M. (author), Cheng, Z. (author), Qian, K. (author), Verhallen, T.W. (author), Wang, C. (author), Wagemaker, M. (author)The development of safe and high-performance Li-metal anodes is crucial to meet the demanded increase in energy density of batteries. However, severe reactivity of Li metal with typical electrolytes and dendrite formation leads to a poor cycle life and safety concerns. Therefore, it is essential to develop electrolytes that passivate the...journal article 2019
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Liu, M. (author), Cheng, Z. (author), Ganapathy, S. (author), Wang, C. (author), Haverkate, Lucas A. (author), Tułodziecki, Michał (author), Unnikrishnan, Sandeep (author), Wagemaker, M. (author)In common hybrid solid electrolytes (HSEs), either the ionic conductivity of the polymer electrolyte is enhanced by the presence of a nanosized inorganic filler, which effectively decrease the glass-transition temperature, or the polymer solid electrolyte acts mostly as a flexible host for the inorganic solid electrolyte, the latter providing...journal article 2019
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Yu, C. (author), Ganapathy, S. (author), van Eck, Ernst R H (author), Wang, H.. (author), Basak, S. (author), Li, Z. (author), Wagemaker, M. (author)Solid-state batteries potentially offer increased lithium-ion battery energy density and safety as required for large-scale production of electrical vehicles. One of the key challenges toward high-performance solid-state batteries is the large impedance posed by the electrode-electrolyte interface. However, direct assessment of the lithium...journal article 2017
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Tang, Linkai (author), He, Yan Bing (author), Wang, Chao (author), Wang, Shuan (author), Wagemaker, M. (author), Li, Baohua (author), Yang, Quan Hong (author), Kang, Feiyu (author)Nanosized Li<sub>4</sub>Ti<sub>5</sub>O<sub>12</sub> (LTO) materials enabling high rate performance suffer from a large specific surface area and low tap density lowering the cycle life and practical energy density. Microsized LTO materials have high density which generally compromises their rate capability. Aiming at combining the favorable...journal article 2017
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