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Li, Huanhuan (author), Duan, Peigao (author), Huang, Yawen (author), Cui, Chengsen (author), Hollmann, F. (author), Ma, Yunjian (author), Wang, Yonghua (author), Zhang, Jie (author), Liu, Weidong (author), Zhang, Wuyuan (author)The downstream product transformation of lignin depolymerization is of great interest in the production of high-value aromatic chemicals. However, this transformation is often impeded by chemical oxidation under harsh reaction conditions. In this study, we demonstrate that hypohalites generated in situ by the vanadium-containing...journal article 2024
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Jang, Jinha (author), Aurangzeb Khan, Waseela (author), Hollmann, F. (author), Won, Keehoon (author), Park, Chan Beum (author)Lignin is the most abundant renewable and sustainable source of aromatic compounds to replace fossil resources, causing environmental issues. However, most lignin generated from pulping and biorefinery processes is combusted or discarded as waste. In this work, we first propose a photocatalytic artificial wood platform consisting of lignin and...journal article 2024
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Valero Romero, M.J. (author), García-Mateos, F. J. (author), Kapteijn, F. (author), Rodríguez-Mirasol, J. (author), Cordero, T. (author)Cobalt-containing lignin-based fibers were synthesized in one step by electrospinning of Alcell lignin solutions as carbon precursor, a low-cost and renewable co-product of the paper making industry. The lignin fibers were thermostabilized in air to avoid the fusion during the carbonization process between 500 and 800 °C to obtain cobalt...journal article 2023
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Lin, P. (author), Liu, X. (author), Ren, S. (author), Li, Yi (author), Xu, Jian (author), Li, Mingliang (author)High-Content SBS Polymer Modified Asphalt Mixtures (HCPMA) combined with fibers have gained popularity in porous pavement construction due to their superior performance. Although the aging behavior of HCPMA has been extensively studied, the impact of fibers on performance and aging susceptibility remains unclear. This research investigates the...journal article 2023
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Bierach, C.B. (author), Alberts Coelho, A.A.C. (author), Turrin, M. (author), Așut, Serdar (author), Knaack, U. (author)Under urgent sustainability targets, the building industry craves for renewable and recyclable biomaterials as cellulose is a fiber; Lignin is a plant-derived low-cost polymer with remarkable properties, yet its valorization is in its infancy. Recent studies have shown potentials to combine cellulose and lignin into a renewable bio-based...journal article 2023
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Santana Martin, María (author)Epoxy resins are one of the most relevant and widely used thermosets in the market covering a wide range of applications. Industries are being forced to quickly transition towards sustainable alternatives due to the pressure from emerging environmental concerns, the depletion of petrochemical supplies, and compliance with environmental...master thesis 2022
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Alberts Coelho, Alexsander (author)The building stock and the construction industry combined are responsible for a large share of greenhouse gases emissions. At the same time, every year tons of wood, paper and agricultural residues are wasted instead of recycled and upcycled into the production chain. In the fabrication field, the relevance of additive manufacturing processes is...master thesis 2022
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Bierach, Christopher (author)With a building industry that is responsible for a large amount of our carbon emissions, a rising population, and the over-extraction of resources, architects and engineers have the responsibility to use environmentally friendly products. Lignin and cellulose are the most abundant biopolymers on earth and produce a lot of waste by ending up...master thesis 2022
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Kim, Jinhyun (author), Um, Yunna (author), Han, Seunghyun (author), Hilberath, T. (author), Kim, Yong Hwan (author), Hollmann, F. (author), Park, Chan Beum (author)The pulp and paper manufacturers generate approximately 50 million metric tons of lignin per annum, most of which has been abandoned or incinerated because of lignin's recalcitrant nature. Here, we report bias-free photoelectrochemical (PEC) oxidation of lignin coupled with asymmetric hydrogenation of C=C bonds. The PEC platform consists of a...journal article 2022
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Kumru, B. (author)Solar irradiation provides critical energy to conduct chemical reactions. Many light-sensitive materials, such as semiconductors, guide photoredox-induced chemical pathways to tailor favored chemical conversions. Polymer synthesis by light is popular, however mainly addressed by conducting radical-based polymerization strategies. Oxidative...journal article 2022
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Zhang, Y. (author), Liu, X. (author), Ren, S. (author), Jing, R. (author), Lin, P. (author), Apostolidis, P. (author), Erkens, S. (author), Wang, Xuancang (author), Scarpas, Athanasios (author)Lignin, one of the most abundant natural polymers, has been extensively studied as an additive in bituminous binders. Even though the lignin improves the overall resistance against oxidative aging of bitumen, it could lead to high thermal cracking sensitivity. In this study, a bio-oil (i.e., rapeseed oil) is implemented in lignin-modified...journal article 2022
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Oliveira, Raisa C.P. (author), Buijnsters, J.G. (author), Mateus, Maria M. (author), Bordado, João C.M. (author), Santos, Diogo M.F. (author)Black liquor (BL) is a highly alkaline byproduct from pulp mills. BL is rich in inorganic and organic compounds, with lignin (a natural polymer) being the most abundant. Following a waste biorefinery concept, the electrolysis of BL comprises lignin oxidation at the anode and hydrogen evolution at the cathode. These paired electrochemical...journal article 2022
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Shams, Shams T. (author), Zhang, Jie (author), Tonin, F. (author), Hinderks, Renske (author), Deurloo, Y.N. (author), Urlacher, Vlada B. (author), Hagedoorn, P.L. (author)Lignin valorization may offer a sustainable approach to achieve a chemical industry that is not completely dependent on fossil resources for the production of aromatics. However, lignin is a recalcitrant, heterogeneous, and complex polymeric compound for which only very few catalysts can act in a predictable and reproducible manner. Laccase...journal article 2021
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Ren, S. (author), Liu, X. (author), Zhang, Y. (author), Lin, P. (author), Apostolidis, P. (author), Erkens, S. (author), Li, Mingliang (author), Xu, Jian (author)Lignin, as a major waste from biofuel and paper industries, could be utilized as a modifier to enhance the relevant performance of bitumen. However, the effects of lignin on the thermodynamics properties and molecular structure of bitumen are rarely studied. Meanwhile, the potential modification mechanism of lignin modified bitumen is still...journal article 2021
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Garcia Solano, Magnolia (author)This study explored the interactions between alkaline hydrothermal pretreatment (AHPT) operational conditions temperature (°C), NaOH concentration (M) and residence time (min) on the compositional characteristics of the solid (SH) and liquid hydrolysate (LH) obtained from AHPT of sugarcane bagasse (SCB), empty fruit bunch (EFB) and agave bagasse...master thesis 2020
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Zhang, Y. (author), Liu, X. (author), Apostolidis, P. (author), Jing, R. (author), Erkens, S. (author), Poeran, Natascha (author), Scarpas, Athanasios (author)Organosolv lignin, a natural polymer, has been used in this study as an oxidation inhibitor in bitumen. Particularly, the effect of oxidative aging on the chemical compositional changes and on the rheology of bituminous binders with organosolv lignin and the impact to inhibit oxidation in bitumen were evaluated. Firstly, after analyzing the...journal article 2020
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Zhang, Y. (author), Wang, Xuancang (author), Ji, Guanyu (author), Fan, Zhenyang (author), Guo, Yuchen (author), Gao, Wenze (author), Xin, Lei (author)Lignin, as a bio-based waste, has been utilized in the asphalt industry due to various advantages. This study aimed to investigate the effects of two lignin products (lignin powder and lignin fiber) on the mechanical properties of asphalt mixtures. The raveling, rutting, thermal and fatigue cracking resistance, and moisture susceptibility of...journal article 2020
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Zhang, Yi (author), Liu, X. (author), Apostolidis, P. (author), Gard, W.F. (author), van de Ven, Martin (author), Erkens, S. (author), Jing, R. (author)As bitumen oxidizes, material stiffening and embrittlement occur, and bitumen eventually cracks. The use of anti-oxidants, such as lignin, could be used to delay oxidative aging and to extend the lifetime of asphalt pavements. In this study, the chemical and rheological effect of lignin on bitumen was evaluated by using a single dosage organsolv...journal article 2019
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Romero, Jefferson O. (author), Fernandez Fueyo, E. (author), Avila-Salas, Fabián (author), Recabarren, Rodrigo (author), Alzate-Morales, Jans (author), Martínez, Angel T. (author)Lignin peroxidase (LiP) and its natural substrate veratryl alcohol (VA) play a crucial role in lignin degradation by white-rot fungi. Understanding the molecular determinants for the interaction of this enzyme with its substrates is essential in the rational design of engineered peroxidases for biotechnological application. Here, we combine...journal article 2019
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Vural Gursel, Iris (author), Dijkstra, Jan W. (author), Huijgen, Wouter J.J. (author), Ramirez, Andrea (author)This paper presents a techno-economic assessment of three novel routes for the production of bio-based aromatics from lignin. It aims to provide insights into their feasibility and hotspots at an early stage of development to guide further research and development and to facilitate commercialization. The lignin conversion routes are: (non...journal article 2019
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