Operando Transmission Electron Microscopy Study of All-Solid-State Battery Interface: Redistribution of Lithium among Interconnected Particles

With operando transmission electron microscopy visualizing the solid-solid electrode-electrolyte interface of silicon active particles and lithium oxide solid electrolyte as a model system, we show that (de)lithiation (battery cycling) does not require all particles to be in direct contact with electrolytes across length scales of a few...

Electrochemical stability of the next generation lithium batteries

Batteries gained a lot of attention due to a raising demand for energy storage, as required for renewable energy generation systems, portable electronics and transport applications. For the development of new battery materials understanding of fundamental processes is essential, which often relies on the development of new characterisation...