Operando Transmission Electron Microscopy Study of All-Solid-State Battery Interface: Redistribution of Lithium among Interconnected Particles

With operando transmission electron microscopy visualizing the solid-solid electrode-electrolyte interface of silicon active particles and lithium oxide solid electrolyte as a model system, we show that (de)lithiation (battery cycling) does not require all particles to be in direct contact with electrolytes across length scales of a few...

Evidence of the Griffiths phase in multiferroic BiMnO3 and BiFe0.5Mn0.5O3 films

Microstructure and magnetic properties of BiMnO3 and BiFe0.5Mn0.5O3 films, prepared by rf magnetron sputtering on LaAlO3 (001) single-crystalline substrate, are investigated. The selected-area electron diffraction analysis allows us to identify the crystal structure of the BiMnO3 film as orthorhombic, while the BiFe0.5Mn0.5O3 film has a...

Near field imaging of terahertz focusing onto rectangular apertures

We performed terahertz near-field experiments on single rectangular holes with various lengths grown on an electro-optic crystal substrate with ?/100 resolution. We find that the near-field amplitude becomes proportionally larger as the rectangle becomes narrower, strongly suggesting that a constant energy passes through even for a very narrow...

Fourier-transform terahertz near-field imaging of one-dimensional slit arrays: Mapping of electric-field-, magnetic-field-, and Poynting vectors

We present 2D measurements of the full THz electric field behind a sample consisting of multiple slits in a metal foil. Our measurements, which have a sub-wavelength spatial, and a sub-period temporal resolution, reveal electric field lines, electric field vortices and saddle points. From our measurements we are able to reconstruct the magnetic...