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Schins, J.M. (author)The retrieval of the primary (subpicosecond) photoproducts in small-band two-dimensional time-domain terahertz spectroscopy has succeeded only in a few model systems, due to the complicated correlation between the two time parameters. We show that the nature of the primary photoproducts is revealed upon differentiating the measured time-domain...journal article 2010
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Schins, J.M. (author), Hendry, E. (author), Bonn, M. (author), Muller, H.G. (author)We present an analytical expression for the observed signal in time- and phase-resolved pump-probe studies, with particular emphasis on terahertz time-domain spectroscopy. Maxwell’s equations are solved for the response of damped, harmonic oscillators to a driving probe field in the perturbative regime. Our analytical expressions agree with the...journal article 2007