In this study, the hybridization of flax and silk fibre reinforced composites, at ply level, were studied and compared to their monolithic counterparts. Hybrid FRP laminates were produced via the filmstacking compression moulding method using the highly ductile thermoplastic high-density polyethylene grafted with maleic-anhydride as the matrix. The fibre volume fraction ratio between the two fibres and the lay-up configuration were studied, resulting in hybrid composites with different degrees of distribution of the flax and silk plies within the laminate. The results showed that more balanced properties in terms of stiffness, strength, strain to failure, and impact energy absorption can be achieved by varying those two parameters, thus increasing the designing freedom tailored to specific engineering applications. Additionally, the findings revealed that by optimizing those parameters, multiple fractures of the flax plies or “fragmentation” can be achieved as a toughening mechanism, leading to a pseudo-ductile hybrid composite with a gradual or delayed failure development. The fibre fragmentation mechanism, apart from the increased ductility, can be potentially used as a failure detection criterion for structural health monitoring.@en