Comparative analysis of carbon dioxide and hydrogen plume migration in aquifers inspired by the FluidFlower benchmark study

Journal Article (2025)
Author(s)

A. Misaghi Bonabi (TU Delft - Numerical Analysis)

W.A. van Rooijen (TU Delft - Reservoir Engineering)

M.S.K. Al Kobaisi (TU Delft - Numerical Analysis)

Cornelis Vuik (TU Delft - Delft Institute of Applied Mathematics)

H. Hajibeygi (TU Delft - Reservoir Engineering)

Research Group
Numerical Analysis
DOI related publication
https://doi.org/10.1016/j.ijhydene.2025.04.401
More Info
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Publication Year
2025
Language
English
Research Group
Numerical Analysis
Volume number
135
Pages (from-to)
56-68
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Abstract

Large-scale geological storages of hydrogen (H2) and carbon dioxide (CO2) in saline aquifers present feasible options for a sustainable energy future. We compared the plume migration of CO2 and H2 in aquifers using the FluidFlower benchmark, incorporating the state-of-the-art thermophysical and petrophysical properties. The H2 plume, with its higher buoyancy and mobility compared to CO2, remains predominantly in the gas phase due to its lower solubility, increasing the chances of escaping through fractures or migration to distant regions. This additionally leads to a higher pressurized reservoir, which, along with higher buoyancy, increases the chance of caprock penetration. Dissolution trapping of CO2 into brine increases over time due to its fingering, while H2 does not show fingering. Our findings show that while geological carbon storage (GCS) benefits significantly from all structural, dissolution, and residual trapping, underground hydrogen storage (UHS) relies mainly on structural trapping, making the integrity of sealing elements of the system a key factor in its performance.