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van Dijk, Raymond (author), Kalisvaart, D. (author), Cnossen, J.P. (author), Smith, C.S. (author)Single-molecule localization microscopy requires sparse activation of emitters to circumvent the diffraction limit. In densely labeled or thick samples, overlap of emitter images is inevitable. Single-molecule localization of these samples results in a biased parameter estimate with a wrong model of the number of emitters. On the other hand,...journal article 2023
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Almajed, Hussain M. (author), Guerra, Omar J. (author), Smith, W.A. (author), Hodge, Bri Mathias (author), Somoza Tornos, A. (author)Defossilizing the chemical industry using air-to-chemical processes offers a promising solution to driving down the emission trajectory to net-zero by 2050. Syngas is a key intermediate in the chemical industry, which can be produced from electrolytic H2 and air-sourced CO2. To techno-economically assess possible emerging air-to-syngas routes,...journal article 2023
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Li, Q. (author), Finn, Adrian J. (author), Doyle, Stephen J. (author), Smith, Robin (author), Kiss, A.A. (author)This paper explores the basis on which reliable screening of distillation sequences for energy-efficient separation of zeotropic multicomponent mixtures can be carried out. A case study for the separation of natural gas liquids is used to demonstrate the approach. To solve this generic problem, a screening algorithm has been developed using...journal article 2023
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van Hattem, A. (author), Vlieland, J. (author), Dankelman, B.J.R. (author), Thijs, M.A. (author), Wallez, Gilles (author), Dardenne, Kathy (author), Rothe, Jörg (author), Konings, R. (author), Smith, A.L. (author)The quaternary compound Cs<sub>2</sub>Pb(MoO<sub>4</sub>)<sub>2</sub> was synthesized and its structure was characterized using X-ray and neutron diffraction from 298 to 773 K, while thermal expansion was studied from 298 to 723 K. The crystal structure of the high-temperature phase β-Cs<sub>2</sub>Pb(MoO<sub>4</sub>)<sub>2</sub> was...journal article 2023
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Mahler, M.S. (author), Malone Portu, L.M. (author), van den Berg, D.F. (author), Smith, Leah M. (author), Brouns, S.J.J. (author), Fineran, Peter C. (author)Serratia sp. ATCC 39006 is a Gram-negative bacterium that has been used to study the function of phage defences, such as CRISPR-Cas, and phage counter-defence mechanisms. To expand our phage collection to study the phage-host interaction with Serratia sp. ATCC 39006, we isolated the T4-like myovirus LC53 in Ōtepoti Dunedin, Aotearoa New...journal article 2023
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Nagalingam, Nagaraj (author), Raghunathan, Aswin (author), Korede, V.B. (author), Overmars, E.F.J. (author), Hung, S. (author), Hartkamp, Remco (author), Padding, J.T. (author), Smith, C.S. (author), Eral, H.B. (author)Optofluidic devices have revolutionized the manipulation and transportation of fluid at smaller length scales ranging from micrometers to millimeters. We describe a dedicated optical setup for studying laser-induced cavitation inside a microchannel. In a typical experiment, we use a tightly focused laser beam to locally evaporate the solution...journal article 2023
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van Hattem, A. (author), Griveau, Jean Christophe (author), Colineau, Eric (author), Lefering, A.J.E. (author), Konings, R. (author), Smith, A.L. (author)The heat capacities of CsPbI<sub>3</sub>, Cs<sub>4</sub>PbI<sub>6</sub>, and Cs<sub>3</sub>Bi<sub>2</sub>I<sub>9</sub> were studied using low-temperature thermal relaxation calorimetry in the temperature range of 1.9-300 K. The three compounds are insulators, with no electronic contribution to the heat capacity. None of them show detectable...journal article 2023
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van Velde, P.F. (author), Rieger, B. (author), Hinsdale, T.A. (author), Cnossen, J.P. (author), Fan, D. (author), Hung, S. (author), Grunwald, D. (author), Smith, C.S. (author)Three dimensional modulation-enhanced single-molecule localization techniques, such as ModLoc, offer advancements in axial localization precision across the entire field of view and axial capture range, by applying phase shifting to the illumination pattern. However, this improvement is limited by the pitch of the illumination pattern that...journal article 2023
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Glielmo, Luigi (author), Grammatico, S. (author), Kebriaei, Hamed (author), Smith, Roy S. (author)Editorialcontribution to periodical 2023
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Hung, S. (author), Llobet Rosell, Arnau (author), Jurriens, Daphne (author), Soloviev, O.A. (author), Kapitein, Lukas C. (author), Grußmayer, K.S. (author), Neukomm, Lukas J. (author), Verhaegen, M.H.G. (author), Smith, C.S. (author)Single-molecule localization microscopy (SMLM) enables the high-resolution visualization of organelle structures and the precise localization of individual proteins. However, the expected resolution is not achieved in tissue as the imaging conditions deteriorate. Sample-induced aberrations distort the point spread function (PSF), and high...journal article 2022
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Wiersma, M.S.J. (author), Heiles, B.G. (author), Kalisvaart, D. (author), Maresca, D. (author), Smith, C.S. (author)Ultrasound localization microscopy (ULM) is a vascular imaging method that provides a 10-fold improvement in resolution compared to ultrasound Doppler imaging. Because typical ULM acquisitions accumulate large numbers of synthetic microbubble (MB) trajectories over hundreds of cardiac cycles, transient hemodynamic variations such as pulsatility...journal article 2022
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Xia, P. (author), Vercruysse, F. (author), Celada-Casero, Carola (author), Verleysen, P. (author), Petrov, R.H. (author), Sabirov, I. (author), Molina-Aldareguia, J. M. (author), Smith, A. (author), Linke, B. (author), Frometa, D. (author)The article focuses on the effect of alloying and microstructure on formability of advanced high strength steels (AHSSs) processed via quenching and partitioning (Q&P). Three different Q&P steels with different combination of alloying elements and volume fraction of retained austenite are subjected to uniaxial tensile and Nakajima...journal article 2022
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Chandrashekar, S. (author), Iglesias van Montfort, H.P. (author), Bohra, D. (author), Filonenko, G.A. (author), Geerlings, J.J.C. (author), Burdyny, T.E. (author), Smith, W.A. (author)The specific identity of electrolyte cations has many implications in various electrochemical reactions. However, the exact mechanism by which cations affect electrochemical reactions is not agreed upon in the literature. In this report, we investigate the role of cations during the electrochemical reduction of CO2 by chelating the cations...journal article 2022
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Ripepi, D. (author), Izelaar, B. (author), van Noordenne, D.D. (author), Jungbacker, M.P. (author), Kolen, M. (author), Karanth, P. (author), Cruz, Daniel (author), Zeller, Patrick (author), Pérez-Dieste, Virginia (author), Villar-Garcia, Ignacio J. (author), Smith, W.A. (author), Mulder, F.M. (author)Hydrogen permeable electrodes can be utilized for electrolytic ammonia synthesis from dinitrogen, water, and renewable electricity under ambient conditions, providing a promising route toward sustainable ammonia. The understanding of the interactions of adsorbing N and permeating H at the catalytic interface is a critical step toward the...journal article 2022
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Kalisvaart, D. (author), Cnossen, J.P. (author), Hung, S. (author), Stallinga, S. (author), Verhaegen, M.H.G. (author), Smith, C.S. (author)Modulation enhanced single-molecule localization microscopy (meSMLM) methods improve the localization precision by using patterned illumination to encode additional position information. Iterative meSMLM (imeSMLM) methods iteratively generate prior information on emitter positions, used to locally improve the localization precision during...journal article 2022
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Smith, A.L. (author)Molten salts have recently received increased attention worldwide as key materials for sustainable and low-carbon energy supply technologies (e.g. thermal energy storage, concentrated solar power technologies, fission and fusion nuclear reactors) thanks to their appealing thermo-physical properties. In particular, they are used as fuel and...review 2022
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Sassenburg, M. (author), Kelly, Maria (author), Subramanian, S.S. (author), Smith, W.A. (author), Burdyny, T.E. (author)Salt precipitation is a problem in electrochemical CO2 reduction electrolyzers that limits their long-term durability and industrial applicability by reducing the active area, causing flooding and hindering gas transport. Salt crystals form when hydroxide generation from electrochemical reactions interacts homogeneously with CO2 to generate...journal article 2022
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Miller, S.R.M. (author), Smith, Marcus (author)This article considers individual rights and fundamental tenets of the criminal justice system in the context of DNA evidence, in particular recent advancements in genomics that have significantly advanced law enforcement investigative capabilities in this area. It discusses a technique known as Investigative Genetic Genealogy (IGG) which...journal article 2022
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Cai, Yifan (author), Dahiya, Abhinav (author), Wilde, N. (author), Smith, Stephen L. (author)In this paper, we consider the problem of allocating human operator assistance in a system with multiple autonomous robots. Each robot is required to complete independent missions, each defined as a sequence of tasks. While executing a task, a robot can either operate autonomously or be teleoperated by the human operator to complete the task at...conference paper 2022
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Dutta, Shamak (author), Wilde, N. (author), Smith, Stephen L. (author)We present a new mixed integer formulation for the discrete informative path planning problem in random fields. The objective is to compute a budget constrained path while collecting measurements whose linear estimate results in minimum error over a finite set of prediction locations. The problem is known to be NP-hard. However, we strive to...conference paper 2022