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B.J. Cook

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Observing atomic motions as they occur is the dream goal of ultrafast electron microscopy (UEM). Great progress has been made so far thanks to the efforts of many scientists in developing the photoemission sources and beam blankers needed to create short pulses of electrons for the UEM experiments. While details on these setups have typically been reported, a systematic overview of methods used to obtain a pulsed beam and a comparison of relevant source parameters have not yet been conducted. In this report, we outline the basic requirements and parameters that are important for UEM. Different types of imaging modes in UEM are analyzed and summarized. After reviewing and analyzing the different kinds of photoemission sources and beam blankers that have been reported in the literature, we estimate the reduced brightness for all the photoemission sources reviewed and compare this to the brightness in the continuous and blanked beams. As for the problem of pulse broadening caused by the repulsive forces between electrons, four main methods available to mitigate the dispersion are summarized. We anticipate that the analysis and conclusions provided in this manuscript will be instructive for designing an UEM setup and could thus push the further development of UEM. ...
Journal article (2016) - Ben Cook, Pieter Kruit
Photofield emitters show great potential for many single electron pulsed applications. However, for the brightest pulses > 10 11 A / (m 2 sr V), our simulations show that Poisson statistics and stochastic Coulomb interactions limit the brightness and increase the energy spread even with an average of a single electron per pulse. For the systems, we study we find that the energy spread is probably the limiting factor for most applications. ...