P.N. Meza Ramos
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Although numerous projects worldwide have shown encouraging results, landfill stabilization remains challenged by the inherent heterogeneity of the waste body. This complexity limits uniform treatment and leaves uncertainties about the physical, chemical, and biological interactions at play. Addressing these knowledge gaps, this thesis investigates the effectiveness of aeration and water recirculation in three Dutch pilot landfills: Braambergen and Wieringermeer (aerated), and Kragge (water recirculation).
The pilots revealed that the effects of aeration are highly variable in space and time. At Braambergen, variability in aeration performance revealed the strong influence of site heterogeneity. Differences in water levels in aeration wells affected gas composition and flow, yet high water columns alone could not explain the observed contrast between compartments. Other factors, such as spatial variability in gas permeability within the waste body, also played a role. Where aeration was more effective, higher gas extraction, elevated temperatures, and greater settlement indicated enhanced microbial activity and carbon mineralization.
Beyond gas monitoring, stabilization was assessed by comparing the carbon generation of waste samples under aerobic and anaerobic conditions with model predictions and with carbon actually recovered on-site. The heterogeneity of the waste samples was reflected in the carbon potential and decay rate constants (k-values). Aerated pilots showed reduced aerobic carbon potential, reflecting advanced stabilization, while the recirculated pilot retained substantial degradable organic matter. These results highlight both the large potential of aeration to accelerate stabilization and the persistence of heterogeneity that complicates prediction and management.
A further focus was placed on building a comprehensive carbon and nitrogen balance across the solid, aqueous, and gas phases at field scale. Over seven years, aerated pilots exhibited higher organic matter degradation than the anaerobic pilot with a significant share of carbon and nitrogen released through the gas phase. In contrast, the recirculated pilot retained larger amounts of degradable carbon and poorly mobilizable nitrogen. Importantly, the analysis revealed that a substantial fraction of nitrogen remains fixed in solid or microbial pools, potentially delaying compliance with leachate emission targets.
Taken together, these findings advance understanding of how aeration and water recirculation influence landfill stabilization. They demonstrate the benefits of aeration for accelerating degradation while also underlining the challenges posed by spatial variability and persistent nitrogen pools. Such insights are crucial for improving the design and implementation of in-situ stabilization strategies and for reducing the long-term aftercare needs of landfills. ...
Although numerous projects worldwide have shown encouraging results, landfill stabilization remains challenged by the inherent heterogeneity of the waste body. This complexity limits uniform treatment and leaves uncertainties about the physical, chemical, and biological interactions at play. Addressing these knowledge gaps, this thesis investigates the effectiveness of aeration and water recirculation in three Dutch pilot landfills: Braambergen and Wieringermeer (aerated), and Kragge (water recirculation).
The pilots revealed that the effects of aeration are highly variable in space and time. At Braambergen, variability in aeration performance revealed the strong influence of site heterogeneity. Differences in water levels in aeration wells affected gas composition and flow, yet high water columns alone could not explain the observed contrast between compartments. Other factors, such as spatial variability in gas permeability within the waste body, also played a role. Where aeration was more effective, higher gas extraction, elevated temperatures, and greater settlement indicated enhanced microbial activity and carbon mineralization.
Beyond gas monitoring, stabilization was assessed by comparing the carbon generation of waste samples under aerobic and anaerobic conditions with model predictions and with carbon actually recovered on-site. The heterogeneity of the waste samples was reflected in the carbon potential and decay rate constants (k-values). Aerated pilots showed reduced aerobic carbon potential, reflecting advanced stabilization, while the recirculated pilot retained substantial degradable organic matter. These results highlight both the large potential of aeration to accelerate stabilization and the persistence of heterogeneity that complicates prediction and management.
A further focus was placed on building a comprehensive carbon and nitrogen balance across the solid, aqueous, and gas phases at field scale. Over seven years, aerated pilots exhibited higher organic matter degradation than the anaerobic pilot with a significant share of carbon and nitrogen released through the gas phase. In contrast, the recirculated pilot retained larger amounts of degradable carbon and poorly mobilizable nitrogen. Importantly, the analysis revealed that a substantial fraction of nitrogen remains fixed in solid or microbial pools, potentially delaying compliance with leachate emission targets.
Taken together, these findings advance understanding of how aeration and water recirculation influence landfill stabilization. They demonstrate the benefits of aeration for accelerating degradation while also underlining the challenges posed by spatial variability and persistent nitrogen pools. Such insights are crucial for improving the design and implementation of in-situ stabilization strategies and for reducing the long-term aftercare needs of landfills.
Within the framework of the Dutch sustainable landfill project iDS, four compartments of the Dutch landfill Braambergen have been treated by in-situ aeration since 2017. The aeration infrastructure comprises 230 wells with a spacing of 15 to 20 m, distrib-uted over an area of around 10 ha, intercepting a waste body of 1.2 × 106 t of contam-inated soils, soil treatment residues, bottom ashes and construction and demolition waste. The wells, used in an alternating fashion for air injection and gas extraction, can also be used to monitor water tables within the waste body. In order to describe the spatial variability of waste hydraulics, design a larger scale leachate pumping test and, eventually, support model predictions of the site’s water balance and emission potential, analyses of leachate composition and pumping tests on individual wells have been conducted. The spatial variability of leachate quality and water tables is very high with no geospatial relationship between the sampling points. Each sampling point is representative of itself only. Large differences prevail not only between and across the compartments, but also between directly neighbouring wells. Both the small scale differences in leachate tables as well as in leachate quality indicate a spatial pattern of zones with low horizontal connectivity within the waste body. Recovery rates of drawdown in the wells yielded preliminary estimates of horizontal waste hydraulic conductivity in the order of 1×10-7 to 6×10-4 m/s.
In-situ aeration of landfills accelerates biodegradation of waste organic matter and hence advances waste stabilization. The spatial outreach of aeration greatly affects stabilization efficiency. This study analyzed the spatial variability of gas composition and flow in 230 wells spread over four compartments of a Dutch landfill which is under in situ aeration since 2017, as well as the carbon extraction efficiency, tem-perature, and settlement. Flow rates and gas composition in the extraction wells varied strongly. The highest variability was observed in the compartment with the highest water tables with submerged filter screens for most wells, with low flow rates, and elevated ratios of CH4 to CO2, indicating predominance of anaerobic processes (compartment 11Z). The compartment with the most uniform distribution of gas flow rates, composition and lower ratios of CH4 to CO2, suggesting a significant share of aerobic carbon mineralization, also showed higher temperatures, a carbon extraction efficiency, and larger cumulative settlement, all indicative of enhanced microbial activity (compartment 11N). In this compartment, the amount of extracted carbon exceeded the carbon generation predicted from landfill gas modeling by the factor of 2 over the hitherto four years aeration. The effect of water tables on gas flow and the correlation between the flow, and the ratio of CH4 to CO2 appeared weak, indicating that also other factors than water tables influence gas concentration and flow. Future work includes stable isotope probing to analyze the significance of microbial respiration and microbial CH4 oxidation for the composition of the final extracted gas mixture.