In 1911, Heike Kamerlingh Onnes and his research team measured a steep drop to zero in the resistance of mercury when cooling it below4.2 K: superconductivity was discovered. Forty-six years later, the microscopic theory to describe superconductivity was formulated. It predicts that disorder (the increase of electron scattering due to impurities, defects or other causes), to first order, does not influence the superconducting state. From an application perspective, disordered superconductors are interesting as they have a high kinetic inductance: they strongly - and non-linearly - oppose the change in current due to the inertia of the superconducting charge carriers, which are paired electrons, or Cooper pairs. Therefore, disordered superconductors can be used in superconducting circuits as highly inductive, nonlinear elements to realize, for example, quantum bits, quantum-limited amplifiers and single-photon detectors. In addition, the high normal state resistance of disordered superconductors allows an efficient, broadband absorption of light, which enables single photon counting, energy resolving microwave kinetic inductance detectors (MKIDs) for visible and near-infrared light.
These applications are, however, hindered by an unexplained microwave loss and, for MKID applications, an enhanced decay rate of the elementary excitations in the superconductor. Both these effects become stronger with increasing disorder. The elementary excitations are called quasiparticles and are essentially broken Cooper pairs. Their density decays as they recombine pair-wise into Cooper pairs. Since quasiparticles also induce microwave loss, these observations point towards an effect of disorder on the quasiparticle dynamics. It is however unclear how disorder affects the quasiparticle dynamics exactly.....

Disordered superconductors offer new impedance regimes for quantum circuits, enable a pathway to protected qubits, and can improve superconducting detectors due to their high kinetic inductance and sheet resistance. The performance of these devices can be limited, however, by quasiparticles—the fundamental excitations of a superconductor. While experiments have shown that disorder affects the relaxation of quasiparticles drastically, the microscopic mechanisms are still not understood. We address this issue by measuring quasiparticle relaxation in a disordered β-Ta film, which we pattern as the inductor of a microwave resonator. We observe that quasiparticle recombination is governed by the phonon scattering time, which is faster than conventional recombination in ordered superconductors. We interpret the results as recombination of localized quasiparticles, induced by disorder, which first delocalize via phonon absorption. We analyze quasiparticle relaxation measurements on superconductors with different degrees of disorder and conclude that this phenomenon is inherent to disordered superconductors.

Parallel-plate capacitors (PPC) significantly reduce the size of superconducting microwave resonators, reducing the pixel pitch for arrays of single-photon energy-resolving kinetic inductance detectors (KIDs). The frequency noise of KIDs is typically limited by tunneling two-level systems (TLS), which originate from lattice defects in the dielectric materials required for PPCs. How the frequency noise level depends on the PPC's dimensions has not been experimentally addressed. We measure the frequency noise of 56 resonators with a-SiC:H PPCs, which cover a factor of 44 in PPC area and a factor of 4 in dielectric thickness. To support the noise analysis, we measure the resonators' TLS-induced power-dependent intrinsic loss and temperature-dependent resonance frequency shift. From the TLS models, we expect a geometry-independent microwave loss and resonance frequency shift, which is set by the TLS properties of the dielectric. However, we observe a thickness-dependent microwave loss and resonance frequency shift; this is explained by surface layers that limit the performance of PPC-based resonators. For a uniform dielectric, the frequency noise level should scale directly inversely with the PPC area and thickness. We observe that an increase in PPC size reduces the frequency noise, but the exact scaling is, in some cases, weaker than expected. Finally, we derive engineering guidelines for the design of KIDs based on PPC-based resonators.

Kinetic inductance detectors (KIDs) are superconducting energy-resolving detectors, sensitive to single photons from the near-infrared to ultraviolet. We study a hybrid KID design consisting of a β-phase tantalum (β-Ta) inductor and a Nb-Ti-N interdigitated capacitor. The devices show an average intrinsic quality factor Qi of 4.3×105±1.3×105. To increase the power captured by the light-sensitive inductor, we 3D print an array of 150×150μm resin microlenses on the backside of the sapphire substrate. The shape deviation between design and printed lenses is smaller than 1μm, and the alignment accuracy of this process is δx=+5.8±0.5μm and δy=+8.3±3.3μm. We measure a resolving power for 1545-402 nm that is limited to 4.9 by saturation in the KID's phase response. We can model the saturation in the phase response with the evolution of the number of quasiparticles generated by a photon event. An alternative coordinate system that has a linear response raises the resolving power to 5.9 at 402 nm. We verify the measured resolving power with a two-line measurement using a laser source and a monochromator. We discuss several improvements that can be made to the devices on a route towards KID arrays with high resolving powers.

A noiseless, photon-counting detector, which resolves the energy of each photon, could radically change astronomy, biophysics, and quantum optics. Superconducting detectors promise an intrinsic resolving power at visible wavelengths of R=E/δE≈100 due to their low excitation energy. We study superconducting energy-resolving microwave kinetic inductance detectors (MKIDs), which hold particular promise for larger cameras. A visible and near-infrared photon absorbed in the superconductor creates a few thousand quasiparticles through several stages of electron-phonon interaction. Here we demonstrate experimentally that the resolving power of MKIDs at visible to near-infrared wavelengths is limited by the loss of hot phonons during this process. We measure the resolving power of our aluminum-based detector as a function of photon energy using four lasers with wavelengths between 1545-402nm. For detectors on thick SiN/Si and sapphire substrates the resolving power is limited to 10-21 for the respective wavelengths, consistent with the loss of hot phonons. When we suspend the sensitive part of the detector on a 110-nm-thick SiN membrane, the measured resolving power improves to 19-52, respectively. The improvement is equivalent to a factor 8±2 stronger phonon trapping on the membrane, which is consistent with a geometrical phonon propagation model for these hot phonons. We discuss a route towards the Fano limit by phonon engineering.