Spaceborne NO₂ column observations from two high-resolution instruments, Tropospheric Monitoring Instrument (TROPOMI) on board Sentinel-5 Precursor and Ozone Monitoring Instrument (OMI) on Aura, reveal unprecedented NO₂ decreases over China, South Korea, western Europe, and the United States as a result of public health measures enforced to contain the coronavirus disease outbreak (Covid-19) in January–April 2020. The average NO₂ column drop over all Chinese cities amounts to −40% relative to the same period in 2019 and reaches up to a factor of ~2 at heavily hit cities, for example, Wuhan, Jinan, while the decreases in western Europe and the United States are also significant (−20% to −38%). In contrast with this, although Iran is also strongly affected by the disease, the observations do not show evidence of lower emissions, reflecting more limited health measures.

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By applying an inversion algorithm to NO_x satellite observations from Ozone Monitoring Instrument, monthly NO_x emissions for a 10 year period (2007 to 2016) over Chinese seas are presented for the first time. No effective regulations on NO_x emissions have been implemented for ships in China, which is reflected in the trend analysis of maritime emissions. The maritime emissions display a continuous increase rate of about 20% per year until 2012 and slow down to 3% after that. The seasonal cycle of shipping emissions has regional variations, but all regions show lower emissions during winter. Simulations by an atmospheric chemistry transport model show a notable influence of maritime emissions on air pollution over coastal areas, especially in summer. The satellite-derived spatial distribution and the magnitude of maritime emissions over Chinese seas are in good agreement with bottom-up studies based on the Automatic Identification System of ships.

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We present a 3-D climatology of the desert dust distribution over South and East Asia derived using CALIPSO (Cloud-Aerosol Lidar and Infrared Pathfinder Satellite Observation) data. To distinguish desert dust from total aerosol load we apply a methodology developed in the framework of EARLINET (European Aerosol Research Lidar Network). The method involves the use of the particle linear depolarization ratio and updated lidar ratio values suitable for Asian dust, applied to multiyear CALIPSO observations (January 2007-December 2015). The resulting dust product provides information on the horizontal and vertical distribution of dust aerosols over South and East Asia along with the seasonal transition of dust transport pathways. Persistent high D-AOD (dust aerosol optical depth) values at 532 nm, of the order of 0.6, are present over the arid and semi-arid desert regions. Dust aerosol transport (range, height and intensity) is subject to high seasonality, with the highest values observed during spring for northern China (Taklimakan and Gobi deserts) and during summer over the Indian subcontinent (Thar Desert). Additionally, we decompose the CALIPSO AOD (aerosol optical depth) into dust and non-dust aerosol components to reveal the nondust AOD over the highly industrialized and densely populated regions of South and East Asia, where the non-dust aerosols yield AOD values of the order of 0.5. Furthermore, the CALIPSO-based short-term AOD and D-AOD time series and trends between January 2007 and December 2015 are calculated over South and East Asia and over selected subregions. Positive trends are observed over northwest and east China and the Indian subcontinent, whereas over southeast China trends are mostly negative. The calculated AOD trends agree well with the trends derived from Aqua MODIS (Moderate Resolution Imaging Spectroradiometer), although significant differences are observed over specific regions.

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We designed a fast procedure to detect the nitrogen oxides (NOx) sources in the China North Plain and to estimate their NOx emissions through a two-dimensional Gaussian fitting method applied to averaged Ozone Monitoring Instrument (OMI) observations of nitrogen dioxide (NO2) column concentration. The Northern China Plain is a region that has one of the highest densities of anthropogenic NOx sources in the world and therefore the sources are difficult to distinguish. With our procedure we still found 94 individual NOx emission sources. Of these sources Tangshan city has the strongest NOx emission rate (92 Gg N year—1), while the weakest that we are still able to detect is Zhangjiakou city, with a NOx emission rate of 0.4 Gg N year—1. Using the fitting results, we reconstruct the NO2 column concentration distribution map, which matches the OMI observations with an R2 = 0.85 and a slope of 0.78. The derived NOx emission rates for cities and provinces level show good agreement with former studies.@en

We compare nine emission inventories of nitrogen oxides including four satellite-derived NO_x inventories and the following bottom-up inventories for East Asia: REAS (Regional Emission inventory in ASia), MEIC (Multiresolution Emission Inventory for China), CAPSS (Clean Air Policy Support System) and EDGAR (Emissions Database for Global Atmospheric Research). Two of the satellitederived inventories are estimated by using the DECSO (Daily Emission derived Constrained by Satellite Observations) algorithm, which is based on an extended Kalman filter applied to observations from OMI or from GOME-2. The other two are derived with the EnKF algorithm, which is based on an ensemble Kalman filter applied to observations of multiple species using either the chemical transport model CHASER and MIROC-chem. The temporal behaviour and spatial distribution of the inventories are compared on a national and regional scale. A distinction is also made between urban and rural areas. The intercomparison of all inventories shows good agreement in total NO_x emissions over mainland China, especially for trends, with an average bias of about 20% for yearly emissions. All the inventories show the typical emission reduction of 10% during the Chinese New Year and a peak in December. Satellite-derived approaches using OMI show a summer peak due to strong emissions from soil and biomass burning in this season. Biases in NO_x emissions and uncertainties in temporal variability increase quickly when the spatial scale decreases. The analyses of the differences show the importance of using observations from multiple instruments and a high spatial resolution model for the satellite-derived inventories, while for bottom-up inventories, accurate emission factors and activity information are required. The advantage of the satellite-derived approach is that the emissions are soon available after observation, while the strength of the bottom-up inventories is that they include detailed information of emissions for each source category.

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We improve the emission estimate algorithm DECSO (Daily Emission estimates Constrained by Satellite Observations) to better detect NO_x emissions over remote areas. The new version is referred to as DECSO v5. The error covariance of the sensitivity of NO₂ column observations to gridded NO_x emissions has been better characterized. This reduces the background noise of emission estimates by a factor of 10. An emission update constraint has been added to avoid unrealistic day-to-day fluctuations of emissions. We estimate total NO_x emissions, which include biogenic emissions that often drive the seasonal cycle of the NO_x emissions. We demonstrate the improvements implemented in DECSO v5 for the domain of East Asia in the year 2012 and 2013. The emissions derived by DECSO v5 are in good agreement with other inventories like MIX. In addition, the improved algorithm is able to better capture the seasonality of NO_x emissions and for the first time it reveals ship tracks near the Chinese coasts that are otherwise hidden by the outflow of NO₂ from the Chinese mainland. The precision of monthly emissions derived by DECSO v5 for each grid cell is about 20%.

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