Developing effective global strategies for climate mitigation requires an independent assessment of the greenhouse gas emission inventory at the urban scale. In the framework of the Dutch Ruisdael Observatory infrastructure project, we have enhanced the Dutch Atmospheric Large-Eddy-Simulation (DALES) model to simulate carbon dioxide (CO2) plume emission and three-dimensional dispersion within the turbulent boundary layer. The unique ability to explicitly resolve turbulent structures a the hectometer resolution (100 m) makes DALES particularly suitable for detailed realistic simulations of both singular high-emitting point sources and urban emissions, aligning with the goals of Ruisdael Observatory. The model setup involves a high-resolution simulation (100 m × 100 m) covering the main urban area of the Netherlands (51.5–52.5° N, 3.75–6.45° E). The model integrates meteorological forcing from the HARMONIE-AROME weather forecasting model, background CO2 levels from the CAMS reanalysis, and point source emissions and downscaled area emissions derived from the 1 km × 1 km emission inventory from the national registry. The latter are prepared using a sector-specific downscaling workflow, covering major emission categories. Biogenic CO2 exchanges from grasslands and forests are interactively included in the hectometer calculations within the heterogeneous land–surface model of DALES. Our evaluation strategy is twofold, comparing DALES simulations with (i) the state-of-the art LOTOS-EUROS model simulations and (ii) Ruisdael surface observations of the urban background in the Rotterdam area at Westmaas and Slufter and in situ rural Cabauw tower measurements. Our comprehensive statistical analysis confirmed the effectiveness of DALES at modeling the urban-scale CO2 emission distribution and plume dispersion under turbulent conditions but also revealed potential limitations and areas for further improvement. Thus, our new model framework provides valuable insights into the role of anthropogenic and biogenic contributions to local CO2 levels, as well as the transport and dispersion of CO2 emissions. This supports emission uncertainty reduction using atmospheric measurements and contributes to the development of effective regional climate mitigation strategies.

Numerical simulations of the tropical mesoscales often exhibit a self-reinforcing feedback between cumulus convection and shallow circulations, which leads to the self-aggregation of clouds into large clusters. We investigate whether this basic feedback can be adequately captured by large-eddy simulations (LESs). To do so, we simulate the non-precipitating, cumulus-topped boundary layer of the canonical “BOMEX” case over a range of numerical settings in two models. Since the energetic convective scales underpinning the self-aggregation are only slightly larger than typical LES grid spacings, aggregation timescales do not converge even at rather high resolutions (<100 m). Therefore, high resolutions or improved sub-filter scale models may be required to faithfully represent certain forms of trade-wind mesoscale cloud patterns and self-aggregating deep convection in large-eddy and cloud-resolving models, and to understand their significance relative to other processes that organize the tropical mesoscales.

In polar regions, where the boundary layer is often stably stratified, atmospheric models produce large biases depending on the boundary-layer parametrizations and the parametrization of the exchange of energy at the surface. This model intercomparison focuses on the very stable stratification encountered over the Antarctic Plateau in 2009. Here, we analyze results from 10 large-eddy-simulation (LES) codes for different spatial resolutions over 24 consecutive hours, and compare them with observations acquired at the Concordia Research Station during summer. This is a challenging exercise for such simulations since they need to reproduce both the 300-m-deep convective boundary layer and the very thin stable boundary layer characterized by a strong vertical temperature gradient (10 K difference over the lowest 20 m) when the sun is low over the horizon. A large variability in surface fluxes among the different models is highlighted. The LES models correctly reproduce the convective boundary layer in terms of mean profiles and turbulent characteristics but display more spread during stable conditions, which is largely reduced by increasing the horizontal and vertical resolutions in additional simulations focusing only on the stable period. This highlights the fact that very fine resolution is needed to represent such conditions. Complementary sensitivity studies are conducted regarding the roughness length, the subgrid-scale turbulence closure as well as the resolution and domain size. While we find little dependence on the surface-flux parametrization, the results indicate a pronounced sensitivity to both the roughness length and the turbulence closure.