Efficient Continuous Light-Driven Electrochemical Water Splitting Enabled by Monolithic Perovskite-Silicon Tandem Photovoltaics

Journal Article (2022)
Author(s)

Kunal Datta (Eindhoven University of Technology)

Bruno Branco (Eindhoven University of Technology)

Yifeng Zhao (TU Delft - Photovoltaic Materials and Devices)

Valerio Zardetto (DIANA FEA )

Nga Phung (Eindhoven University of Technology)

Andrea Bracesco (Eindhoven University of Technology)

Luana Mazzarella (TU Delft - Photovoltaic Materials and Devices)

Martijn M. Wienk (Eindhoven University of Technology)

Olindo Isabella (TU Delft - Photovoltaic Materials and Devices)

undefined More Authors (External organisation)

DOI related publication
https://doi.org/10.1002/admt.202201131 Final published version
More Info
expand_more
Publication Year
2022
Language
English
Issue number
2
Volume number
8 (2023)
Article number
2201131
Downloads counter
335
Collections
Institutional Repository
Reuse Rights

Other than for strictly personal use, it is not permitted to download, forward or distribute the text or part of it, without the consent of the author(s) and/or copyright holder(s), unless the work is under an open content license such as Creative Commons.

Abstract

Solar-assisted water electrolysis is a promising technology for storing the energy of incident solar irradiation into hydrogen as a fuel. Here, an integrated continuous flow electrochemical reactor coupled to a monolithic perovskite-silicon tandem solar cell is demonstrated that provides light-driven electrochemical solar-to-hydrogen conversion with an energy conversion efficiency exceeding 21% at 1-Sun equivalent light intensity and stable operation during three simulated day-night cycles.