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Martinez-Rabert, Eloi (author), van Amstel, Chiel (author), Smith, Cindy (author), Sloan, William T. (author), Gonzalez Cabaleiro, R. (author)In microbial communities, the ecological interactions between species of different populations are responsible for the spatial distributions observed in aggregates (granules, biofilms or flocs). To explore the underlying mechanisms that control these processes, we have developed a mathematical modelling framework able to describe, label and...journal article 2022
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Kolen, M. (author), Ripepi, D. (author), Smith, W.A. (author), Burdyny, T.E. (author), Mulder, F.M. (author)The nitrogen reduction reaction (NRR) is a promising pathway toward the decarbonization of ammonia (NH3) production. However, unless practical challenges related to the detection of NH3 are removed, confidence in published data and experimental throughput will remain low for experiments in aqueous electrolyte. In this perspective, we analyze...journal article 2022
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Venugopal, A. (author), Egberts, Laurentius H.T. (author), Meeprasert, J. (author), Pidko, E.A. (author), Dam, B. (author), Burdyny, T.E. (author), Sinha, V. (author), Smith, W.A. (author)Finding alternative ways to tailor the electronic properties of a catalyst to actively and selectively drive reactions of interest has been a growing research topic in the field of electrochemistry. In this Letter, we investigate the tuning of the surface electronic properties of electrocatalysts via polymer modification. We show that when a...journal article 2022
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Smith, C.G. (author), Shepherd, Jami (author), Renaud, G.G.J. (author), van Wijk, Kasper (author)By changing the ultrasonic receiving angle in post-processing, we can obtain flow vectors from a photoacoustic experiment on a blood vessel phantom by solving the photoacoustic Doppler equation using a least-squares optimisation approach.conference paper 2022
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Burdyny, T.E. (author), Sassenburg, M. (author), de Rooij, R. (author), Nessbit, Nathan (author), Kas, R. (author), Chandrashekar, S. (author), Firet, N.J. (author), Yang, K. (author), Liu, K. (author), Blommaert, M.A. (author), Kolen, M. (author), Ripepi, D. (author), Smith, W.A. (author)Continued advancements in the electrochemical reduction of CO 2 (CO 2RR) have emphasized that reactivity,selectivity, and stability are not explicit material properties butcombined effects of the catalyst, double-layer, reaction environ-<br/>ment, and system configuration. These realizations have steadily built upon the foundational work...journal article 2022
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Mc Cluskey, K.A. (author), van Veen, E.N.W. (author), Cnossen, J.P. (author), Wesselink, W.J. (author), Asscher, F.M. (author), Smith, C.S. (author), Dekker, N.H. (author)Accurate image alignment is critical in multicolor single-molecule fluorescence microscopy. Global alignment using affine transformations leaves residual errors due to the nonlinearity of the distortions, which decreases the effective field of view. Subsequent local refinement demands either large amounts of reference data and processing time...journal article 2021
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Hung, S. (author), Cnossen, J.P. (author), Fan, D. (author), Smith, C.S. (author)Optical sectioning technologies achieve high precision localization by reducing the background photon count. We use tilted light-sheet microscopy to achieve optical sectioning in localization microscopy, enabling thick sample observation and low background photon count images. A deformable mirror was incorporated to generate a tetrapod point...conference paper 2021
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Ocadiz flores, J.A. (author), Gheribi, A. E. (author), Vlieland, J. (author), Dardenne, K. (author), Rothe, J. (author), Konings, R. (author), Smith, A.L. (author)© 2021 The Authors LiF-UF4 is a key binary system for molten fluoride reactor technology, which has not been scrutinized as thoroughly as the closely related LiF-ThF4 system. The phase diagram equilibria in the system LiF-UF4 are explored in this work with X-ray diffraction (XRD) and differential scanning calorimetry (DSC). The short-range...journal article 2021
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Smith, Marcus (author), Miller, S.R.M. (author)Genomic data is growing in importance as scientific knowledge and technology develop, and in availability, as direct-to-consumer genomic health testing and recreational genealogy services become more widely utilized. Access to genomic data needs to be considered in light of individual privacy. Cross-sector use of genomic health and ancestry data...journal article 2021
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van Oudenaren, G. I.L. (author), Ocadiz flores, J.A. (author), Smith, A.L. (author)Molten chloride salts are ionic liquids in which the anions and cations exhibit network formation. An attractive salt system for use in molten salt reactors is NaCl-UCl<sub>3</sub>, an ionic liquid with complex non-ideal thermodynamic behaviour due to the formation of short-range order. The relationship between local structure and...journal article 2021
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Smith, Marcus (author), Miller, S.R.M. (author)Biometric facial recognition is an artificial intelligence technology involving the automated comparison of facial features, used by law enforcement to identify unknown suspects from photographs and closed circuit television. Its capability is expanding rapidly in association with artificial intelligence and has great potential to solve crime...journal article 2021
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Ocadiz flores, J.A. (author), Rooijakkers, B.A.S. (author), Konings, R. (author), Smith, A.L. (author)The ACl-ThCl (Formula presented.) (A = Li, Na, K) systems could be of relevance to the nuclear industry in the near future. A thermodynamic investigation of the three binary systems is presented herein. The excess Gibbs energy of the liquid solutions is described using the quasi-chemical formalism in the quadruplet approximation. The phase...journal article 2021
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Vermillion, Chris (author), Cobb, Mitchell (author), Fagiano, Lorenzo (author), Leuthold, Rachel (author), Diehl, Moritz (author), Smith, Roy S. (author), Wood, Tony A. (author), Rapp, S. (author), Schmehl, R. (author)Airborne wind energy systems convert wind energy into electricity using tethered flying devices, typically flexible kites or aircraft. Replacing the tower and foundation of conventional wind turbines can substantially reduce the material use and, consequently, the cost of energy, while providing access to wind at higher altitudes. Because the...review 2021
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Nesbitt, N.T. (author), Smith, W.A. (author)Electrochemical atomic force microscopy (EC-AFM) enables measurement of electrode topography and mechanical properties during electrochemical reactions. However, for aqueous-based reactions that make gas products, such as CO2 reduction and water splitting into CO/H2, current densities below 1 mA cm-2 have been necessary to prevent formation...journal article 2021
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- Buonsanti, Raffaella (author), Smith, W.A. (author) journal article 2021
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Mitchell, Jessica (author), Smith, C.S. (author), Titlow, Josh (author), Otto, Nils (author), van Velde, P.F. (author), Booth, Martin (author), Davis, Ilan (author), Waddell, Scott (author)Memory-relevant neuronal plasticity is believed to require local translation of new proteins at synapses. Understanding this process requires the visualization of the relevant mRNAs within these neuronal compartments. Here, we used single-molecule fluorescence in situ hybridization to localize mRNAs at subcellular resolution in the adult...journal article 2021
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- Batista, Victor (author), Li, Can (author), Smith, W.A. (author), Wang, Dunwei (author) contribution to periodical 2021
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Assessing Silver Palladium Alloys for Electrochemical CO2 Reduction in Membrane Electrode AssembliesChandrashekar, S. (author), Geerlings, J.J.C. (author), Smith, W.A. (author)The field of electrochemical CO<sub>2</sub> reduction has been transitioning to industrially relevant scales by changing the architecture of the electrochemical cells and moving away from the traditional aqueous H-cells to membrane electrode assemblies (MEA). The reaction environments in MEAs vary drastically from that of aqueous H-cells,...journal article 2021
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Blommaert, M.A. (author), Subramanian, S.S. (author), Yang, K. (author), Smith, W.A. (author), Vermaas, D.A. (author)Typically, anion exchange membranes (AEMs) are used in CO2 electrolyzers, but those suffer from unwanted CO2 crossover, implying (indirect) energy consumption for generating an excess of CO2 feed and purification of the KOH anolyte. As an alternative, bipolar membranes (BPMs) have been suggested, which mitigate the reactant loss by...journal article 2021
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Smith, C.S. (author), Slotman, Johan A. (author), Schermelleh, Lothar (author), Chakrova, N. (author), Hari, S. (author), Vos, Y. (author), Hagen, C.W. (author), Houtsmuller, A.B. (author), Hoogenboom, J.P. (author), Stallinga, S. (author)Super-resolution structured illumination microscopy (SIM) has become a widely used method for biological imaging. Standard reconstruction algorithms, however, are prone to generate noise-specific artifacts that limit their applicability for lower signal-to-noise data. Here we present a physically realistic noise model that explains the...journal article 2021