Nanophotonics with Diamond Color Centers: Quantum Optics and Entanglement Protocols

A large-scale quantum network, where many nodes are connected via entanglement and can share and process quantum information, will allow applications that are now unattainable. While some are known, ranging from distributed quantum computing to enhanced quantum sensing and quantum communication, the full potential of such a fundamentally new...

Filtering and Imaging of Frequency-Degenerate Spin Waves Using Nanopositioning of a Single-Spin Sensor

Nitrogen-vacancy (NV) magnetometry is a new technique for imaging spin waves in magnetic materials. It detects spin waves by their microwave magnetic stray fields, which decay evanescently on the scale of the spin-wavelength. Here, we use nanoscale control of a single-NV sensor as a wavelength filter to characterize frequency-degenerate spin...

Imaging Spin-Wave Damping Underneath Metals Using Electron Spins in Diamond

Spin waves in magnetic insulators are low-damping signal carriers that can enable a new generation of spintronic devices. The excitation, control, and detection of spin waves by metal electrodes is crucial for interfacing these devices to electrical circuits. As such, it is important to understand metal-induced damping of spin-wave transport,...

Investigating the possible origin of Raman bands in defective sp2/sp3 carbons below 900 cm−1: Phonon density of states or double resonance mechanism at play?

Multiwavelength Raman spectroscopy (325, 514, 633 nm) was used to analyze three different kinds of samples containing sp2 and sp3 carbons: chemical vapor deposited diamond films of varying microstructure, a plasma-enhanced chemical vapor deposited hydrogenated amorphous carbon film heated at 500 °C and highly oriented pyrolytic graphite exposed...

Optimal design of diamond-air microcavities for quantum networks using an analytical approach

Defect centres in diamond are promising building blocks for quantum networks thanks to a long-lived spin state and bright spin-photon interface. However, their low fraction of emission into a desired optical mode limits the entangling success probability. The key to overcoming this is through Purcell enhancement of the emission. Open Fabry...

Experimental Investigation of Adhesion and Friction Phenomena of Ultrananocrystalline Diamond (UNCD) and Aluminum Oxide in MEMS

This thesis aims to provide the latest progresses on the experimental investigation of friction and adhesion phenomena, occurring at the nanoscale in microelectromechanical systems (MEMS). I have studied and characterized the interaction between MEMS sidewalls in contact and sliding one onto another. Ultrananocrystalline diamond (UNCD) and...

Hydrogen termination of CVD diamond films by high-temperature annealing at atmospheric pressure

A high-temperature procedure to hydrogenate diamond films using molecular hydrogen at atmospheric pressure was explored. Undoped and doped chemical vapour deposited (CVD) polycrystalline diamond films were treated according to our annealing method using a H2 gas flow down to ?50 ml/min (STP) at ?850?°C. The films were extensively evaluated by...

Current-induced nanogap formation and graphitization in boron-doped diamond films

A high-current annealing technique is used to fabricate nanogaps and hybrid diamond/graphite structures in boron-doped nanocrystalline diamond films. Nanometer-sized gaps down to ?1?nm are produced using a feedback-controlled current annealing procedure. The nanogaps are characterized using scanning electron microscopy and electronic transport...

Quantum control and coherence of interacting spins in diamond

The field of quantum science and technology has generated many ideas for new revolutionary devices that exploit the quantum mechanical properties of small-scale systems. Isolated solid state spins play a large role in quantum technologies. They can be used as basic building blocks for a quantum computer or as ultra-sensitive magnetic-field...

Quantum control of single spins and single photons in diamond

This thesis describes a series of experiments on the control of the optical properties of the nitrogen-vacancy (NV) center in diamond, and on control of the electron and nuclear spin states associated with the NV center. The NV center is a fluorescing atomic defect center in diamond, consisting of a substitutional nitrogen atom adjacent to a...

Deterministic nanoassembly of a coupled quantum emitter–photonic crystal cavity system

Controlling the interaction of a single quantum emitter with its environment is a key challenge in quantum optics. Here, we demonstrate deterministic coupling of single nitrogen-vacancy (NV) centers to high-quality photonic crystal cavities. We preselect single NV centers and position their 50-nm-sized host nanocrystals into the mode maximum of...

Nanopositioning of a diamond nanocrystal containing a single nitrogen-vacancy defect center

Precise control over the position of a single quantum object is important for many experiments in quantum science and nanotechnology. We report on a technique for high-accuracy positioning of individual diamond nanocrystals. The positioning is done with a home-built nanomanipulator under real-time scanning electron imaging, yielding an accuracy...

Generation and transport of photoexcited electrons in single-crystal diamond

We report time-dependent photocurrent and transport measurements of sub-bandgap photoexcited carriers in nitrogen-rich (type Ib), single-crystal diamond. Transient carrier dynamics are characteristic of trapping conduction with long charge storage lifetimes of ? 3?hours. By measuring the photoexcited Hall effect, we confirm that the charge...

Single atom doping for quantum device development in diamond and silicon

The ability to inject dopant atoms with high spatial resolution, flexibility in dopant species, and high single ion detection fidelity opens opportunities for the study of dopant fluctuation effects and the development of devices in which function is based on the manipulation of quantum states in single atoms, such as proposed quantum computers....

High precision form cruch profiling of diamond grinding wheels