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Val Zwiller

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Scaling superconducting nanowire single-photon detectors for imaging at the quantum-limit

Review (2025) - Jun Gao, Jin Chang, Bruno Lopez-Rodriguez, Iman Esmaeil Zadeh, Val Zwiller, Ali W. Elshaari
Superconducting nanowire single-photon detectors (SNSPDs) have emerged as essential devices that push the boundaries of photon detection with unprecedented sensitivity, ultrahigh timing precision, and broad spectral response. Recent advancements in materials engineering, superconducting electronics integration, and cryogenic system design are enabling the evolution of SNSPDs from single-pixel detectors toward scalable arrays and large-format single-photon time tagging cameras. This perspective article surveys the rapidly evolving technological landscape underpinning this transition, focusing on innovative superconducting materials, advanced multiplexed read-out schemes, and emerging cryo-compatible electronics. We highlight how these developments are set to profoundly impact diverse applications, including quantum communication networks, deep-tissue biomedical imaging, single-molecule spectroscopy, remote sensing with unprecedented resolution, and the detection of elusive dark matter signals. By critically discussing both current challenges and promising solutions, we aim to articulate a clear, coherent vision for the next generation of SNSPD-based quantum imaging systems. ...
Journal article (2025) - H. Wang, N. Noordzij, M. Mykhaylov, Stephan Steinhauer, Thomas Descamps, Eitan Oksenberg, Val Zwiller, I.Z. Esmaeil Zadeh
Due to stringent thermal budgets in cryogenic technologies such as superconducting quantum computers and sensors, electronic building blocks that simultaneously offer low energy consumption, fast switching, low error rates, a small footprint, and simple fabrication are pivotal for large-scale devices. Here, we demonstrate a superconducting switch with attojoule switching energy, high speed (pico-second rise/fall times), and high integration density (on the order of 10 -2 μm 2 per switch). It consists of a superconducting nanochannel and a metal heater separated by an insulating silica layer. We experimentally demonstrate digital gate operations utilizing these nanostructures, such as NOT, NAND, NOR, AND, and OR gates, with a few femtojoules of energy consumption and ultralow bit error rates <10 -8. In addition, we build energy-efficient volatile memory elements with nanosecond operation speeds and a retention time over 10 5 s. These superconducting switches open new possibilities for increasing the size and complexity of modern cryogenic technologies. ...
Journal article (2024) - J. W.Niels Los, Mariia Sidorova, Bruno Lopez-Rodriguez, Patrick Qualm, Jin Chang, Stephan Steinhauer, Val Zwiller, Iman Esmaeil Zadeh
Since their first demonstration in 2001 [Gol’tsman et al., Appl. Phys. Lett. 79, 705-707 (2001)], superconducting-nanowire single-photon detectors (SNSPDs) have witnessed two decades of great developments. SNSPDs are the detector of choice in most modern quantum optics experiments and are slowly finding their way into other photon-starved fields of optics. Until now, however, in nearly all experiments, SNSPDs were used as “binary” detectors, meaning that they could only distinguish between 0 and > = 1 photons, and photon number information was lost. Recent research has demonstrated proof-of-principle photon-number resolution (PNR) SNSPDs counting 2-5 photons. The photon-number-resolving capability is highly demanded in various quantum-optics experiments, including Hong-Ou-Mandel interference, photonic quantum computing, quantum communication, and non-Gaussian quantum state preparation. In particular, PNR detectors at the wavelength range of 850-950 nm are of great interest due to the availability of high-quality semiconductor quantum dots (QDs) [Heindel et al., Adv. Opt. Photonics 15, 613-738 (2023)] and high-performance cesium-based quantum memories [Ma et al., J. Opt. 19, 043001 (2017)]. In this paper, we demonstrate NbTiN-based SNSPDs with >94% system detection efficiency, sub-11 ps timing jitter for one photon, and sub-7 ps for 2 photons. More importantly, our detectors resolve up to 7 photons using conventional cryogenic electric readout circuitry. Through theoretical analysis, we show that the PNR performance of demonstrated detectors can be further improved by enhancing the signal-to-noise ratio and bandwidth of our readout circuitry. Our results are promising for the future of optical quantum computing and quantum communication. ...
Review (2023) - Jin Chang, Jun Gao, Iman Esmaeil Zadeh, Ali W. Elshaari, Val Zwiller
At the core of quantum photonic information processing and sensing, two major building pillars are single-photon emitters and single-photon detectors. In this review, we systematically summarize the working theory, material platform, fabrication process, and game-changing applications enabled by state-of-the-art quantum dots in nanowire emitters and superconducting nanowire single-photon detectors. Such nanowire-based quantum hardware offers promising properties for modern quantum optics experiments. We highlight several burgeoning quantum photonics applications using nanowires and discuss development trends of integrated quantum photonics. Also, we propose quantum information processing and sensing experiments for the quantum optics community, and future interdisciplinary applications. ...
Journal article (2023) - Thomas Hummel, Alex Widhalm, Jan Philipp Höpker, Klaus D. Jöns, Jin Chang, Andreas Fognini, Stephan Steinhauer, Val Zwiller, Artur Zrenner, Tim J. Bartley
Superconducting nanowire single-photon detectors (SNSPDs) show near unity efficiency, low dark count rate, and short recovery time. Combining these characteristics with temporal control of SNSPDs broadens their applications as in active de-latching for higher dynamic range counting or temporal filtering for pump-probe spectroscopy or LiDAR. To that end, we demonstrate active gating of an SNSPD with a minimum off-to-on rise time of 2.4 ns and a total gate length of 5.0 ns. We show how the rise time depends on the inductance of the detector in combination with the control electronics. The gate window is demonstrated to be fully and freely, electrically tunable up to 500 ns at a repetition rate of 1.0 MHz, as well as ungated, free-running operation. Control electronics to generate the gating are mounted on the 2.3 K stage of a closed-cycle sorption cryostat, while the detector is operated on the cold stage at 0.8 K. We show that the efficiency and timing jitter of the detector is not altered during the on-time of the gating window. We exploit gated operation to demonstrate a method to increase in the photon counting dynamic range by a factor 11.2, as well as temporal filtering of a strong pump in an emulated pump-probe experiment. ...
Journal article (2022) - Galan Moody, Volker J. Sorger, Daniel J. Blumenthal, Paul W. Juodawlkis, William Loh, Alex E. Jones, Benjamin Pingault, Ali W. Elshaari, Val Zwiller
Integrated photonics will play a key role in quantum systems as they grow from few-qubit prototypes to tens of thousands of qubits. The underlying optical quantum technologies can only be realized through the integration of these components onto quantum photonic integrated circuits (QPICs) with accompanying electronics. In the last decade, remarkable advances in quantum photonic integration have enabled table-top experiments to be scaled down to prototype chips with improvements in efficiency, robustness, and key performance metrics. These advances have enabled integrated quantum photonic technologies combining up to 650 optical and electrical components onto a single chip that are capable of programmable quantum information processing, chip-to-chip networking, hybrid quantum system integration, and high-speed communications. In this roadmap article, we highlight the status, current and future challenges, and emerging technologies in several key research areas in integrated quantum photonics, including photonic platforms, quantum and classical light sources, quantum frequency conversion, integrated detectors, and applications in computing, communications, and sensing. With advances in materials, photonic design architectures, fabrication and integration processes, packaging, and testing and benchmarking, in the next decade we can expect a transition from single- and few-function prototypes to large-scale integration of multi-functional and reconfigurable devices that will have a transformative impact on quantum information science and engineering. ...
Conference paper (2022) - Bruno Lopez Rodriguez, Jin Chang, Johannes W.N. Los, Stephan Steinhauer, Val Zwiller, Iman Esmaeil Zadeh
Ultra-high system detection efficiency (SDE) s uperconducting nanowire single-photon detectors are demonstrated for a broad range of wavelengths, from UV to mid-infrared, opening novel possibilities in the fields of quantum photonics, neuroimaging and astronomy. ...
Journal article (2022) - Jin Chang, Johannes W.N. Los, Ronan Gourgues, Stephan Steinhauer, S. N. Dorenbos, Silvania F. Pereira, H. Paul Urbach, Val Zwiller, Iman Esmaeil Zadeh
Shortly after their inception, superconducting nanowire single-photon detectors (SNSPDs) became the leading quantum light detection technology. With the capability of detecting single-photons with near-unity efficiency, high time resolution, low dark count rate, and fast recovery time, SNSPDs outperform conventional single-photon detection techniques. However, detecting lower energy single photons (<0.8 eV) with high efficiency and low timing jitter has remained a challenge. To achieve unity internal efficiency at mid-infrared wavelengths, previous works used amorphous superconducting materials with low energy gaps at the expense of reduced time resolution (close to a nanosecond), and by operating them in complex milliKelvin (mK) dilution refrigerators. In this work, we provide an alternative approach with SNSPDs fabricated from 5 to 9.5 nm thick NbTiN superconducting films and devices operated in conventional Gifford-McMahon cryocoolers. By optimizing the superconducting film deposition process, film thickness, and nanowire design, our fiber-coupled devices achieved >70% system detection efficiency (SDE) at 2 μm and sub-15 ps timing jitter. Furthermore, detectors from the same batch demonstrated unity internal detection efficiency at 3 μm and 80% internal efficiency at 4 μm, paving the road for an efficient mid-infrared single-photon detection technology with unparalleled time resolution and without mK cooling requirements. We also systematically studied the dark count rates (DCRs) of our detectors coupled to different types of mid-infrared optical fibers and blackbody radiation filters. This offers insight into the trade-off between bandwidth and DCRs for mid-infrared SNSPDs. To conclude, this paper significantly extends the working wavelength range for SNSPDs made from polycrystalline NbTiN to 1.5-4 μm, and we expect quantum optics experiments and applications in the mid-infrared range to benefit from this far-reaching technology. ...
Journal article (2021) - Artur Branny, Pierre Didier, Julien Zichi, Iman Esmaeil Zahed, Stephan Steinhauer, Val Zwiller, Ulrich Vogt
We characterized the performance of abiased superconducting nanowire to detect X-ray photons. The device, made of a 10 nm thin NbTiN film and fabricated on a dielectric substrate (SiO2, Nb3O5) detected 1000 times larger signal than anticipated from direct X-ray absorption. We attributed this effect to X-ray induced generation of secondary particles in the substrate. The enhancement corresponds to an increase in the flux by the factor of 3.6, relative to a state-of-the-art commercial X-ray silicon drift detector. The detector exhibited 8.25 ns temporal recovery time and 82 ps timing resolution, measured using optical photons. Our results emphasize the importance of the substrate in superconducting X-ray single photon detectors. ...
Journal article (2021) - J. Chang, J. W.N. Los, S. N. Dorenbos, I. Esmaeil Zadeh, J. O. Tenorio-Pearl, N. Noordzij, R. Gourgues, A. Guardiani, J. R. Zichi, S. F. Pereira, H. P. Urbach, V. Zwiller
Single photon detectors are indispensable tools in optics, from fundamental measurements to quantum information processing. The ability of superconducting nanowire single photon detectors (SNSPDs) to detect single photons with unprecedented efficiency, short dead time, and high time resolution over a large frequency range enabled major advances in quantum optics. However, combining near-unity system detection efficiency (SDE) with high timing performance remains an outstanding challenge. In this work, we fabricated novel SNSPDs on membranes with 99.5-2.07+0.5% SDE at 1350 nm with 32 ps timing jitter (using a room-temperature amplifier), and other detectors in the same batch showed 94%-98% SDE at 1260-1625 nm with 15-26 ps timing jitter (using cryogenic amplifiers). The SiO2/Au membrane enables broadband absorption in small SNSPDs, offering high detection efficiency in combination with high timing performance. With low-noise cryogenic amplifiers operated in the same cryostat, our efficient detectors reach a timing jitter in the range of 15-26 ps. We discuss the prime challenges in optical design, device fabrication, and accurate and reliable detection efficiency measurements to achieve high performance single photon detection. As a result, the fast developing fields of quantum information science, quantum metrology, infrared imaging, and quantum networks will greatly benefit from this far-reaching quantum detection technology. ...

A perspective on evolution, state-of-the-art, future developments, and applications

Journal article (2021) - Iman Esmaeil Zadeh, J. Chang, Johannes W.N. Los, Samuel Gyger, Ali W. Elshaari, Stephan Steinhauer, Sander N. Dorenbos, Val Zwiller
Two decades after their demonstration, superconducting nanowire single-photon detectors (SNSPDs) have become indispensable tools for quantum photonics as well as for many other photon-starved applications. This invention has not only led to a burgeoning academic field with a wide range of applications but also triggered industrial efforts. Current state-of-the-art SNSPDs combine near-unity detection efficiency over a wide spectral range, low dark counts, short dead times, and picosecond time resolution. The present perspective discusses important milestones and progress of SNSPDs research, emerging applications, and future challenges and gives an outlook on technological developments required to bring SNSPDs to the next level: a photon-counting, fast time-tagging imaging, and multi-pixel technology that is also compatible with quantum photonic integrated circuits. ...
Journal article (2021) - Ali W. Elshaari, Anas Skalli, Samuel Gyger, Martin Nurizzo, Lucas Schweickert, Iman Esmaeil Zadeh, Mikael Svedendahl, Stephan Steinhauer, Val Zwiller
Hybrid integration provides an important avenue for incorporating atom-like solid-state single-photon emitters into photonic platforms that possess no optically-active transitions. Hexagonal boron nitride (hBN) is particularly interesting quantum emitter for hybrid integration, as it provides a route for room-temperature quantum photonic technologies, coupled with its robustness and straightforward activation. Despite the recent progress of integrating hBN emitters in photonic waveguides, a deterministic, site-controlled process remains elusive. Here, the integration of selected hBN emitter in silicon nitride waveguide is demonstrated. A small misalignment angle of 4° is shown between the emission-dipole orientation and the waveguide propagation direction. The integrated emitter maintains high single-photon purity despite subsequent encapsulation and nanofabrication steps, delivering quantum light with zero delay second order correlation function (Formula presented.). The results provide an important step toward deterministic, large scale, quantum photonic circuits at room temperature using atom-like single-photon emitters. ...
Journal article (2020) - Iman Esmaeil Zadeh, Jin Chang, Yuri J. Van Staaden, Jeroen P.E. Swens, Sergiy Dobrovolskiy, Dennis R. Schaart, Silvania F. Pereira, Val Zwiller, Sander N. Dorenbos, More Authors...
A broad range of scientific and industrial disciplines require precise optical measurements at very low light levels. Single-photon detectors combining high efficiency and high time resolution are pivotal in such experiments. By using relatively thick films of NbTiN (8-11 nm) and improving the pattern fidelity of the nanostructure of the superconducting nanowire single-photon detectors (SNSPD), we fabricated devices demonstrating superior performance over all previously reported detectors in the combination of efficiency and time resolution. Our findings prove that small variations in the nanowire width, in the order of a few nanometers, can lead to a significant penalty on their temporal response. Addressing these issues, we consistently achieved high time resolution (best device 7.7 ps, other devices a10-16 ps) simultaneously with high system detection efficiencies (80-90%) in the wavelength range of 780-1000 nm, as well as in the telecom bands (1310-1550 nm). The use of thicker films allowed us to fabricate large-area multipixel devices with homogeneous pixel performance. We first fabricated and characterized a 100 × 100 μm2 16-pixel detector and showed there was little variation among individual pixels. Additionally, to showcase the power of our platform, we fabricated and characterized 4-pixel multimode fiber-coupled detectors and carried out photon-correlation experiments on a nanowire quantum dot resulting in g2(0) values lower than 0.04. The multipixel detectors alleviate the need for beamsplitters and can be used for higher order correlations with promising prospects not only in the field of quantum optics, but also in bioimaging applications, such as fluorescence microscopy and positron emission tomography. ...
Journal article (2020) - Ali W. Elshaari, Adrian Iovan, Samuel Gyger, Iman Esmaeil Zadeh, Julien Zichi, Lily Yang, Stephan Steinhauer, Val Zwiller
We use dispersion engineering to control the signal propagation speed in the feed lines of superconducting single-photon detectors. Using this technique, we demonstrate time-division-multiplexing of two-pixel detectors connected with a slow-RF transmission line, all realized using planar geometry requiring a single lithographic step. Through studying the arrival time of detection events in each pixel vs the fabricated slow-RF coplanar waveguide length, we extract a delay of 1.7 ps per 1 μm of propagation, corresponding to detection signal speeds of ∼0.0019c. Our results open an important avenue to explore the rich ideas of dispersion engineering and metamaterials for superconducting detector applications. ...

Wavelength-resolved Purcell enhancement of PbS/CdS quantum dots measured on a chip-based platform

Conference paper (2020) - Lukas Elsinger, Ronan Gourgues, Iman E. Zadeh, Jorick Maes, Antonio Guardiani, Gabriele Bulgarini, Silvania F. Pereira, Sander N. Dorenbos, Val Zwiller, More authors...
Future quantum optical networks will require an integrated solution to multiplex suitable sources and detectors on a low-loss platform. Here we combined superconducting single-photon detectors with colloidal PbS/CdS quantum dots (QDs) and low-loss silicon nitride passive photonic components to show their combined operation at cryogenic temperatures. Using a planar concave grating spectrometer, we performed wavelength-resolved measurements of the photoluminescence decay of QDs, which were deterministically placed in the gap of plasmonic antennas, in order to improve their emission rate. We observed a Purcell enhancement matching the antenna simulations, with a concurrent increase of the count rate on the superconducting detectors. ...
Conference paper (2019) - Iman Esmaeil Zadeh, Ali Elshaari, Val Zwiller, Silvania Pereira, Johannes W.N. Los, Ronan Gourgues, Julien Zichi, Sander Dorenbos, Michael E. Reimer, Dan Dalacu, Philip J. Poole, Klaus Jöns
Single-photon generation, processing, and detection are the three main components of any quantum optical circuit. We present our results on integration of semiconducting nanowire quantum dots, dielectric waveguides, and ultrahigh performance superconducting nanowire single-photon detectors. ...
Journal article (2019) - Julien Zichi, Jin Chang, Stephan Steinhauer, Kristina Von Fieandt, Johannes W.N. Los, Gijs Visser, Nima Kalhor, Iman Esmaeil Zadeh, Val Zwiller, More Authors...
The requirements in quantum optics experiments for high single-photon detection efficiency, low timing jitter, low dark count rate and short dead time have been fulfilled with the development of superconducting nanowire single-photon detectors. Although they offer a detection efficiency above 90%, achieving a high time resolution in devices made of amorphous materials is a challenge, particularly at temperatures above 0.8 K. Devices made from niobium nitride and niobium titanium nitride allow us to reach the best timing jitter but, in turn, have stronger requirements in terms of film quality to achieve a high efficiency. Here we take advantage of the flexibility of reactive co-sputter deposition to tailor the composition of NbxTi1-xN superconducting films and show that a Nb fraction of x = 0.62 allows for the fabrication of detectors from films as thick as 9 nm and covering an active area of 20 µm, with a wide detection saturation plateau at telecom wavelengths and in particular at 1550 nm. This is a signature of an internal detection efficiency saturation, achieved while maintaining the high time resolution associated with NbTiN and operation at 2.5K. With our optimized recipe, we reliably fabricated detectors with high critical current densities reaching a saturation plateau at 1550 nm with 80% system detection efficiency and with a FWHM timing jitter as low as 19.5 ps. ...
Journal article (2019) - Jin Chang, Iman Esmaeil Zadeh, Johannes W.N. Los, Julien Zichi, Andreas Fognini, Monique Gevers, Sander Dorenbos, Silvania F. Pereira, Paul Urbach, Val Zwiller
In the past decade, superconducting nanowire single-photon detectors (SNSPDs) have gradually become an indispensable part of any demanding quantum optics experiment. Until now, most SNSPDs have been coupled to single-mode fibers. SNSPDs coupled to multimode fibers have shown promising efficiencies but have yet to achieve high time resolution. For a number of applications ranging from quantum nano-photonics to bio-optics, high efficiency and high time resolution are desired at the same time. In this paper, we demonstrate the role of polarization on the efficiency of multimode-fiber-coupled detectors and fabricated high-performance 20 µm, 25 µm, and 50 µm diameter detectors targeted for visible, near-infrared, and telecom wavelengths. A custom-built setup was used to simulate realistic experiments with randomized modes in the fiber. We achieved over 80% system efficiency and <20 ps timing jitter for 20 µm SNSPDs. Also, we realized 70% system efficiency and <20 ps timing jitter for 50 µm SNSPDs. The high-efficiency multimode-fiber-coupled SNSPDs with unparalleled time resolution will benefit various quantum optics experiments and applications in the future. ...
Journal article (2019) - Ronan Gourgues, Johannes W.N. Los, Julien Zichi, Jin Chang, Nima Kalhor, Gabriele Bulgarini, Sander N. Dorenbos, Val Zwiller, Iman Esmaeil Zadeh
We experimentally investigate the performance of NbTiN superconducting nanowire single photon detectors above the base temperature of a conventional Gifford-McMahon cryocooler (2.5 K). By tailoring design and thickness (8 - 13 nm) of the detectors, high performance, high operating temperature, single-photon detection from the visible to telecom wavelengths are demonstrated. At 4.3 K, a detection efficiency of 82 % at 785 nm wavelength and a timing jitter of 30 ± 0.3 ps are achieved. In addition, for 1550 nm and similar operating temperature we measured a detection efficiency as high as 64 %. Finally, we show that at temperatures up to 7 K, unity internal efficiency is maintained for the visible spectrum. Our work is particularly important to allow for the large scale implementation of superconducting single photon detectors in combination with heat sources such as free-space optical windows, cryogenic electronics, microwave sources and active optical components for complex quantum optical experiments and bio-imaging. ...
Journal article (2016) - Ali W. Elshaari, Iman Esmaeil Zadeh, Klaus D. Jöns, Val Zwiller
In this paper, we characterize the Thermo-optic properties of silicon nitride ring resonators between 18 and 300 K. The Thermo-optic coefficients of the silicon nitride core and the oxide cladding are measured by studying the temperature dependence of the resonance wavelengths. The resonant modes show low temperature dependence at cryogenic temperatures and higher dependence as the temperature increases. We find the Thermo-optic coefficients of PECVD silicon nitride and silicon oxide to be 2.51 ± 0.08 E- 5 K-1 and 0.96 ± 0.09 E-5 K-1 at room temperature while decreasing by an order of magnitude when cooling to 18 K. To show the effect of variations in the thermo-optic coefficients on device performance, we study the tuning of a fully integrated electrically tunable filter as a function of voltage for different temperatures. The presented results provide new practical guidelines in designing photonic circuits for studying low-temperature optical phenomena. ...